Colloidal entanglement in highly twisted chiral nematic colloids: Twisted loops, Hopf links, and trefoil knots

The topology and geometry of closed defect loops is studied in chiral nematic colloids with variable chirality. The colloidal particles with perpendicular surface anchoring of liquid crystalline molecules are inserted in a twisted nematic cell with the thickness that is only slightly larger than the...

Full description

Bibliographic Details
Main Authors: Jampani, V, Skarabot, M, Ravnik, M, Copar, S, Zumer, S, Musevic, I
Format: Journal article
Language:English
Published: 2011
_version_ 1797070291274301440
author Jampani, V
Skarabot, M
Ravnik, M
Copar, S
Zumer, S
Musevic, I
author_facet Jampani, V
Skarabot, M
Ravnik, M
Copar, S
Zumer, S
Musevic, I
author_sort Jampani, V
collection OXFORD
description The topology and geometry of closed defect loops is studied in chiral nematic colloids with variable chirality. The colloidal particles with perpendicular surface anchoring of liquid crystalline molecules are inserted in a twisted nematic cell with the thickness that is only slightly larger than the diameter of the colloidal particle. The total twist of the chiral nematic structure in cells with parallel boundary conditions is set to 0, π, 2π, and 3π, respectively. We use the laser tweezers to discern the number and the topology of the -1/2 defect loops entangling colloidal particles. For a single colloidal particle, we observe that a single defect loop is winding around the particle, with the winding pattern being more complex in cells with higher total twist. We observe that colloidal dimers and colloidal clusters are always entangled by one or several -1/2 defect loops. For colloidal pairs in π-twisted cells, we identify at least 17 different entangled structures, some of them exhibiting linked defect loops-Hopf link. Colloidal entanglement is even richer with a higher number of colloidal particles, where we observe not only linked, but also colloidal clusters knotted into the trefoil knot. The experiments are in good agreement with numerical modeling using Landau-de Gennes theory coupled with geometrical and topological considerations using the method of tetrahedral rotation. © 2011 American Physical Society.
first_indexed 2024-03-06T22:36:42Z
format Journal article
id oxford-uuid:5a24e134-77a2-4691-96e5-9fec0c4e8035
institution University of Oxford
language English
last_indexed 2024-03-06T22:36:42Z
publishDate 2011
record_format dspace
spelling oxford-uuid:5a24e134-77a2-4691-96e5-9fec0c4e80352022-03-26T17:14:03ZColloidal entanglement in highly twisted chiral nematic colloids: Twisted loops, Hopf links, and trefoil knotsJournal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:5a24e134-77a2-4691-96e5-9fec0c4e8035EnglishSymplectic Elements at Oxford2011Jampani, VSkarabot, MRavnik, MCopar, SZumer, SMusevic, IThe topology and geometry of closed defect loops is studied in chiral nematic colloids with variable chirality. The colloidal particles with perpendicular surface anchoring of liquid crystalline molecules are inserted in a twisted nematic cell with the thickness that is only slightly larger than the diameter of the colloidal particle. The total twist of the chiral nematic structure in cells with parallel boundary conditions is set to 0, π, 2π, and 3π, respectively. We use the laser tweezers to discern the number and the topology of the -1/2 defect loops entangling colloidal particles. For a single colloidal particle, we observe that a single defect loop is winding around the particle, with the winding pattern being more complex in cells with higher total twist. We observe that colloidal dimers and colloidal clusters are always entangled by one or several -1/2 defect loops. For colloidal pairs in π-twisted cells, we identify at least 17 different entangled structures, some of them exhibiting linked defect loops-Hopf link. Colloidal entanglement is even richer with a higher number of colloidal particles, where we observe not only linked, but also colloidal clusters knotted into the trefoil knot. The experiments are in good agreement with numerical modeling using Landau-de Gennes theory coupled with geometrical and topological considerations using the method of tetrahedral rotation. © 2011 American Physical Society.
spellingShingle Jampani, V
Skarabot, M
Ravnik, M
Copar, S
Zumer, S
Musevic, I
Colloidal entanglement in highly twisted chiral nematic colloids: Twisted loops, Hopf links, and trefoil knots
title Colloidal entanglement in highly twisted chiral nematic colloids: Twisted loops, Hopf links, and trefoil knots
title_full Colloidal entanglement in highly twisted chiral nematic colloids: Twisted loops, Hopf links, and trefoil knots
title_fullStr Colloidal entanglement in highly twisted chiral nematic colloids: Twisted loops, Hopf links, and trefoil knots
title_full_unstemmed Colloidal entanglement in highly twisted chiral nematic colloids: Twisted loops, Hopf links, and trefoil knots
title_short Colloidal entanglement in highly twisted chiral nematic colloids: Twisted loops, Hopf links, and trefoil knots
title_sort colloidal entanglement in highly twisted chiral nematic colloids twisted loops hopf links and trefoil knots
work_keys_str_mv AT jampaniv colloidalentanglementinhighlytwistedchiralnematiccolloidstwistedloopshopflinksandtrefoilknots
AT skarabotm colloidalentanglementinhighlytwistedchiralnematiccolloidstwistedloopshopflinksandtrefoilknots
AT ravnikm colloidalentanglementinhighlytwistedchiralnematiccolloidstwistedloopshopflinksandtrefoilknots
AT copars colloidalentanglementinhighlytwistedchiralnematiccolloidstwistedloopshopflinksandtrefoilknots
AT zumers colloidalentanglementinhighlytwistedchiralnematiccolloidstwistedloopshopflinksandtrefoilknots
AT musevici colloidalentanglementinhighlytwistedchiralnematiccolloidstwistedloopshopflinksandtrefoilknots