Separation of energy scales in the kagome antiferromagnet TmAgGe: A magnetic-field-orientation study up to 55 T

TmAgGe is an antiferromagnet in which the spins are confined to distorted kagome-like planes at low temperatures. We report angle-dependent measurements of the magnetization M in fields of up to 55 T that show that there are two distinct and separate energy scales present in TmAgGe, each responsible...

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Bibliographic Details
Main Authors: Goddard, P, Singleton, J, Sharma, A, Morosan, E, Blundell, S, Bud'ko, S, Canfield, P
Format: Journal article
Language:English
Published: 2007
Description
Summary:TmAgGe is an antiferromagnet in which the spins are confined to distorted kagome-like planes at low temperatures. We report angle-dependent measurements of the magnetization M in fields of up to 55 T that show that there are two distinct and separate energy scales present in TmAgGe, each responsible for a set of step-like metamagnetic transitions: weak exchange interactions and strong crystalline-electric-field (CEF) interactions. Simulations of M using a three-dimensional, free-energy minimization technique allow us to specify the physical origin of the metamagnetic transitions in low, in-plane fields. We also show that the transitions observed with the field perpendicular to the kagome planes are associated with the CEF-split multiplet of Tm. © 2007 The American Physical Society.