Towards higher electron mobility in modulation doped GaAs/AlGaAs core shell nanowires
Precise control over the electrical conductivity of semiconductor nanowires is a crucial prerequisite for implementation into novel electronic and optoelectronic devices. Advances in our understanding of doping mechanisms in nanowires and their influence on electron mobility and radiative efficiency...
| Main Authors: | , , , , , , , |
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| Format: | Journal article |
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Royal Society of Chemistry
2017
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| _version_ | 1797072984660246528 |
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| author | Boland, J Tutuncuoglu, G Gong, J Conesa-Boj, S Davis, C Herz, L Fontcuberta i Morral, A Johnston, M |
| author_facet | Boland, J Tutuncuoglu, G Gong, J Conesa-Boj, S Davis, C Herz, L Fontcuberta i Morral, A Johnston, M |
| author_sort | Boland, J |
| collection | OXFORD |
| description | Precise control over the electrical conductivity of semiconductor nanowires is a crucial prerequisite for implementation into novel electronic and optoelectronic devices. Advances in our understanding of doping mechanisms in nanowires and their influence on electron mobility and radiative efficiency are urgently required. Here, we investigate the electronic properties of n-type modulation doped GaAs/AlGaAs nanowires via optical pump terahertz (THz) probe spectroscopy and photoluminescence spectroscopy over the temperature range 5K-300K. We directly determine an ionisation energy of 6.7±0.5meV (T = 52K) for the Si donors that create the modulation doping in the AlGaAs shell. We further elucidate the temperature dependence of the electron mobility, photoconductivity lifetime and radiative efficiency, and determine the charge-carrier scattering mechanisms that limit electron mobility. We show that below the donor ionization temperature, charge scattering is limited by interactions with interfaces, leading to an excellent electron mobility of 4360±380cm2V-1s-1 at 5 K. Above the ionization temperature, polar scattering via longitudinal optical (LO) phonons dominates, leading to a room temperature mobility of 2220±130cm2V-1s-1. In addition, we show that the Si donors effectively passivate interfacial trap states in the nanowires, leading to prolonged photoconductivity lifetimes with increasing temperature, accompanied by an enhanced radiative efficiency that exceeds 10% at room temperature. |
| first_indexed | 2024-03-06T23:15:34Z |
| format | Journal article |
| id | oxford-uuid:6701e1f6-b5d7-4e1b-8571-851c10cb1395 |
| institution | University of Oxford |
| last_indexed | 2024-03-06T23:15:34Z |
| publishDate | 2017 |
| publisher | Royal Society of Chemistry |
| record_format | dspace |
| spelling | oxford-uuid:6701e1f6-b5d7-4e1b-8571-851c10cb13952022-03-26T18:35:31ZTowards higher electron mobility in modulation doped GaAs/AlGaAs core shell nanowiresJournal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:6701e1f6-b5d7-4e1b-8571-851c10cb1395Symplectic Elements at OxfordRoyal Society of Chemistry2017Boland, JTutuncuoglu, GGong, JConesa-Boj, SDavis, CHerz, LFontcuberta i Morral, AJohnston, MPrecise control over the electrical conductivity of semiconductor nanowires is a crucial prerequisite for implementation into novel electronic and optoelectronic devices. Advances in our understanding of doping mechanisms in nanowires and their influence on electron mobility and radiative efficiency are urgently required. Here, we investigate the electronic properties of n-type modulation doped GaAs/AlGaAs nanowires via optical pump terahertz (THz) probe spectroscopy and photoluminescence spectroscopy over the temperature range 5K-300K. We directly determine an ionisation energy of 6.7±0.5meV (T = 52K) for the Si donors that create the modulation doping in the AlGaAs shell. We further elucidate the temperature dependence of the electron mobility, photoconductivity lifetime and radiative efficiency, and determine the charge-carrier scattering mechanisms that limit electron mobility. We show that below the donor ionization temperature, charge scattering is limited by interactions with interfaces, leading to an excellent electron mobility of 4360±380cm2V-1s-1 at 5 K. Above the ionization temperature, polar scattering via longitudinal optical (LO) phonons dominates, leading to a room temperature mobility of 2220±130cm2V-1s-1. In addition, we show that the Si donors effectively passivate interfacial trap states in the nanowires, leading to prolonged photoconductivity lifetimes with increasing temperature, accompanied by an enhanced radiative efficiency that exceeds 10% at room temperature. |
| spellingShingle | Boland, J Tutuncuoglu, G Gong, J Conesa-Boj, S Davis, C Herz, L Fontcuberta i Morral, A Johnston, M Towards higher electron mobility in modulation doped GaAs/AlGaAs core shell nanowires |
| title | Towards higher electron mobility in modulation doped GaAs/AlGaAs core shell nanowires |
| title_full | Towards higher electron mobility in modulation doped GaAs/AlGaAs core shell nanowires |
| title_fullStr | Towards higher electron mobility in modulation doped GaAs/AlGaAs core shell nanowires |
| title_full_unstemmed | Towards higher electron mobility in modulation doped GaAs/AlGaAs core shell nanowires |
| title_short | Towards higher electron mobility in modulation doped GaAs/AlGaAs core shell nanowires |
| title_sort | towards higher electron mobility in modulation doped gaas algaas core shell nanowires |
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