Mediating Fano losses in plasmonic scatterers by tuning the dielectric environment

Scattering from metal nanoparticles above a high index substrate has the potential to significantly enhance light trapping in thin film devices with minimal additional cost. However, the benefits of this approach are currently limited by short wavelength losses from Fano resonances arising due to in...

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Main Authors: Powell, A, Smith, J
Format: Journal article
Published: AIP Publishing 2016
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author Powell, A
Smith, J
author_facet Powell, A
Smith, J
author_sort Powell, A
collection OXFORD
description Scattering from metal nanoparticles above a high index substrate has the potential to significantly enhance light trapping in thin film devices with minimal additional cost. However, the benefits of this approach are currently limited by short wavelength losses from Fano resonances arising due to interference between the plasmon modes in a nanoparticle. In this paper, the effect of particle-substrate interactions on the observed Fano behaviour is explored in detail, using finite-difference time-domain simulations and an analytical model. Several approaches to mitigate the Fano loss are explored, and it is found that overcoating the particle with a thin dielectric film represents by far the most effective way to remove Fano losses whilst keeping broadband forward scattering high.
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spelling oxford-uuid:77b1abbf-119f-4aae-9e6f-d96db3cc16e22022-03-26T20:25:47ZMediating Fano losses in plasmonic scatterers by tuning the dielectric environmentJournal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:77b1abbf-119f-4aae-9e6f-d96db3cc16e2Symplectic Elements at OxfordAIP Publishing2016Powell, ASmith, JScattering from metal nanoparticles above a high index substrate has the potential to significantly enhance light trapping in thin film devices with minimal additional cost. However, the benefits of this approach are currently limited by short wavelength losses from Fano resonances arising due to interference between the plasmon modes in a nanoparticle. In this paper, the effect of particle-substrate interactions on the observed Fano behaviour is explored in detail, using finite-difference time-domain simulations and an analytical model. Several approaches to mitigate the Fano loss are explored, and it is found that overcoating the particle with a thin dielectric film represents by far the most effective way to remove Fano losses whilst keeping broadband forward scattering high.
spellingShingle Powell, A
Smith, J
Mediating Fano losses in plasmonic scatterers by tuning the dielectric environment
title Mediating Fano losses in plasmonic scatterers by tuning the dielectric environment
title_full Mediating Fano losses in plasmonic scatterers by tuning the dielectric environment
title_fullStr Mediating Fano losses in plasmonic scatterers by tuning the dielectric environment
title_full_unstemmed Mediating Fano losses in plasmonic scatterers by tuning the dielectric environment
title_short Mediating Fano losses in plasmonic scatterers by tuning the dielectric environment
title_sort mediating fano losses in plasmonic scatterers by tuning the dielectric environment
work_keys_str_mv AT powella mediatingfanolossesinplasmonicscatterersbytuningthedielectricenvironment
AT smithj mediatingfanolossesinplasmonicscatterersbytuningthedielectricenvironment