Growth saturation of unstable thin films on transverse-striped hydrophilic-hydrophobic micropatterns

Using three-dimensional numerical simulations, we demonstrate the growth saturation of an unstable thin liquid film on micropatterned hydrophilic-hydrophobic substrates. We consider different transverse-striped micropatterns, characterized by the total fraction of hydrophilic coverage and the width...

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Հիմնական հեղինակներ: Ledesma-Aguilar, R, Hernandez-Machado, A, Pagonabarraga, I
Ձևաչափ: Journal article
Լեզու:English
Հրապարակվել է: 2011
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author Ledesma-Aguilar, R
Hernandez-Machado, A
Pagonabarraga, I
author_facet Ledesma-Aguilar, R
Hernandez-Machado, A
Pagonabarraga, I
author_sort Ledesma-Aguilar, R
collection OXFORD
description Using three-dimensional numerical simulations, we demonstrate the growth saturation of an unstable thin liquid film on micropatterned hydrophilic-hydrophobic substrates. We consider different transverse-striped micropatterns, characterized by the total fraction of hydrophilic coverage and the width of the hydrophilic stripes. We compare the growth of the film on the micropatterns to the steady states observed on homogeneous substrates, which correspond to saturated sawtooth and growing finger configurations for hydrophilic and hydrophobic substrates, respectively. The proposed micropatterns trigger an alternating fingering-spreading dynamics of the film, which leads to a complete suppression of the contact line growth above a critical fraction of hydrophilic stripes. Furthermore, we find that increasing the width of the hydrophilic stripes slows down the advancing front, giving smaller critical fractions the wider the hydrophilic stripes are. Using analytical approximations, we quantitatively predict the growth rate of the contact line as a function of the covering fraction, and predict the threshold fraction for saturation as a function of the stripe width. © The Royal Society of Chemistry 2011.
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spelling oxford-uuid:7b41b937-f697-415c-99be-923d94e5c7a82022-03-26T20:49:22ZGrowth saturation of unstable thin films on transverse-striped hydrophilic-hydrophobic micropatternsJournal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:7b41b937-f697-415c-99be-923d94e5c7a8EnglishSymplectic Elements at Oxford2011Ledesma-Aguilar, RHernandez-Machado, APagonabarraga, IUsing three-dimensional numerical simulations, we demonstrate the growth saturation of an unstable thin liquid film on micropatterned hydrophilic-hydrophobic substrates. We consider different transverse-striped micropatterns, characterized by the total fraction of hydrophilic coverage and the width of the hydrophilic stripes. We compare the growth of the film on the micropatterns to the steady states observed on homogeneous substrates, which correspond to saturated sawtooth and growing finger configurations for hydrophilic and hydrophobic substrates, respectively. The proposed micropatterns trigger an alternating fingering-spreading dynamics of the film, which leads to a complete suppression of the contact line growth above a critical fraction of hydrophilic stripes. Furthermore, we find that increasing the width of the hydrophilic stripes slows down the advancing front, giving smaller critical fractions the wider the hydrophilic stripes are. Using analytical approximations, we quantitatively predict the growth rate of the contact line as a function of the covering fraction, and predict the threshold fraction for saturation as a function of the stripe width. © The Royal Society of Chemistry 2011.
spellingShingle Ledesma-Aguilar, R
Hernandez-Machado, A
Pagonabarraga, I
Growth saturation of unstable thin films on transverse-striped hydrophilic-hydrophobic micropatterns
title Growth saturation of unstable thin films on transverse-striped hydrophilic-hydrophobic micropatterns
title_full Growth saturation of unstable thin films on transverse-striped hydrophilic-hydrophobic micropatterns
title_fullStr Growth saturation of unstable thin films on transverse-striped hydrophilic-hydrophobic micropatterns
title_full_unstemmed Growth saturation of unstable thin films on transverse-striped hydrophilic-hydrophobic micropatterns
title_short Growth saturation of unstable thin films on transverse-striped hydrophilic-hydrophobic micropatterns
title_sort growth saturation of unstable thin films on transverse striped hydrophilic hydrophobic micropatterns
work_keys_str_mv AT ledesmaaguilarr growthsaturationofunstablethinfilmsontransversestripedhydrophilichydrophobicmicropatterns
AT hernandezmachadoa growthsaturationofunstablethinfilmsontransversestripedhydrophilichydrophobicmicropatterns
AT pagonabarragai growthsaturationofunstablethinfilmsontransversestripedhydrophilichydrophobicmicropatterns