Efficient dynamic nuclear polarization at high magnetic fields.

Efficient dynamic nuclear polarization at high magnetic fields.

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By applying a new technique for dynamic nuclear polarization involving simultaneous excitation of electronic and nuclear transitions, we have enhanced the nuclear polarization of the nitrogen nuclei in 15N@C60 by a factor of 10(3) at a fixed temperature of 3 K and a magnetic field of 8.6 T, more tha...

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Príomhchruthaitheoirí: Morley, G, van Tol, J, Ardavan, A, Porfyrakis, K, Zhang, J, Briggs, G
Formáid: Journal article
Teanga:English
Foilsithe / Cruthaithe: 2007
Cur síos
Achoimre:By applying a new technique for dynamic nuclear polarization involving simultaneous excitation of electronic and nuclear transitions, we have enhanced the nuclear polarization of the nitrogen nuclei in 15N@C60 by a factor of 10(3) at a fixed temperature of 3 K and a magnetic field of 8.6 T, more than twice the maximum enhancement reported to date. This methodology will allow the initialization of the nuclear qubit in schemes exploiting N@C60 molecules as components of a quantum information processing device.

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