Magnetic fluctuations and spin freezing in nonsuperconducting LiFeAs derivatives

We present detailed magnetometry and muon-spin rotation data on polycrystalline samples of overdoped, nonsuperconducting LiFe1 -xNixAs (x=0.1,0.2) and Li1-yFe1+yAs (0≤y≤0.04) as well as superconducting LiFeAs. While LiFe1 -xNixAs exhibits weak antiferromagnetic fluctuations down to 1.5K, Li1-yFe1+yA...

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Hoofdauteurs: Wright, J, Pitcher, M, Trevelyan-Thomas, W, Lancaster, T, Baker, P, Pratt, F, Clarke, S, Blundell, S
Formaat: Journal article
Taal:English
Gepubliceerd in: 2013
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author Wright, J
Pitcher, M
Trevelyan-Thomas, W
Lancaster, T
Baker, P
Pratt, F
Clarke, S
Blundell, S
author_facet Wright, J
Pitcher, M
Trevelyan-Thomas, W
Lancaster, T
Baker, P
Pratt, F
Clarke, S
Blundell, S
author_sort Wright, J
collection OXFORD
description We present detailed magnetometry and muon-spin rotation data on polycrystalline samples of overdoped, nonsuperconducting LiFe1 -xNixAs (x=0.1,0.2) and Li1-yFe1+yAs (0≤y≤0.04) as well as superconducting LiFeAs. While LiFe1 -xNixAs exhibits weak antiferromagnetic fluctuations down to 1.5K, Li1-yFe1+yAs samples, which have a much smaller deviation from the 1:1:1 stoichiometry, show a crossover from ferromagnetic to antiferromagnetic fluctuations on cooling and a freezing of dynamically fluctuating moments at low temperatures. We do not find any signatures of time-reversal symmetry breaking in stoichiometric LiFeAs that would support recent predictions of triplet pairing. © 2013 American Physical Society.
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spelling oxford-uuid:86bee1b4-7bc3-445b-bbd6-021c27fd48c32022-03-26T22:06:07ZMagnetic fluctuations and spin freezing in nonsuperconducting LiFeAs derivativesJournal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:86bee1b4-7bc3-445b-bbd6-021c27fd48c3EnglishSymplectic Elements at Oxford2013Wright, JPitcher, MTrevelyan-Thomas, WLancaster, TBaker, PPratt, FClarke, SBlundell, SWe present detailed magnetometry and muon-spin rotation data on polycrystalline samples of overdoped, nonsuperconducting LiFe1 -xNixAs (x=0.1,0.2) and Li1-yFe1+yAs (0≤y≤0.04) as well as superconducting LiFeAs. While LiFe1 -xNixAs exhibits weak antiferromagnetic fluctuations down to 1.5K, Li1-yFe1+yAs samples, which have a much smaller deviation from the 1:1:1 stoichiometry, show a crossover from ferromagnetic to antiferromagnetic fluctuations on cooling and a freezing of dynamically fluctuating moments at low temperatures. We do not find any signatures of time-reversal symmetry breaking in stoichiometric LiFeAs that would support recent predictions of triplet pairing. © 2013 American Physical Society.
spellingShingle Wright, J
Pitcher, M
Trevelyan-Thomas, W
Lancaster, T
Baker, P
Pratt, F
Clarke, S
Blundell, S
Magnetic fluctuations and spin freezing in nonsuperconducting LiFeAs derivatives
title Magnetic fluctuations and spin freezing in nonsuperconducting LiFeAs derivatives
title_full Magnetic fluctuations and spin freezing in nonsuperconducting LiFeAs derivatives
title_fullStr Magnetic fluctuations and spin freezing in nonsuperconducting LiFeAs derivatives
title_full_unstemmed Magnetic fluctuations and spin freezing in nonsuperconducting LiFeAs derivatives
title_short Magnetic fluctuations and spin freezing in nonsuperconducting LiFeAs derivatives
title_sort magnetic fluctuations and spin freezing in nonsuperconducting lifeas derivatives
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AT pitcherm magneticfluctuationsandspinfreezinginnonsuperconductinglifeasderivatives
AT trevelyanthomasw magneticfluctuationsandspinfreezinginnonsuperconductinglifeasderivatives
AT lancastert magneticfluctuationsandspinfreezinginnonsuperconductinglifeasderivatives
AT bakerp magneticfluctuationsandspinfreezinginnonsuperconductinglifeasderivatives
AT prattf magneticfluctuationsandspinfreezinginnonsuperconductinglifeasderivatives
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