Quantifying cloud adjustments and the radiative forcing due to aerosol–cloud interactions in satellite observations of warm marine clouds

<p>Aerosol&ndash;cloud interactions and their resultant forcing remains one of the largest sources of uncertainty in future climate scenarios. The effective radiative forcing due to aerosol&ndash;cloud interactions (ERFaci) is a combination of two different effects, namely how aerosols...

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Bibliographic Details
Main Authors: Douglas, A, L’Ecuyer, T
Format: Journal article
Published: Copernicus Publications 2020
Description
Summary:<p>Aerosol&ndash;cloud interactions and their resultant forcing remains one of the largest sources of uncertainty in future climate scenarios. The effective radiative forcing due to aerosol&ndash;cloud interactions (ERFaci) is a combination of two different effects, namely how aerosols modify cloud brightness (RFaci, intrinsic) and how cloud extent reacts to aerosol (cloud adjustments CA; extrinsic). Using satellite observations of warm clouds from the NASA A-Train constellation from 2007 to 2010 along with MERRA-2 Reanalysis and aerosol from the SPRINTARS model, we evaluate the ERFaci in warm, marine clouds and its components, the RFaci<sub>warm</sub>&nbsp;and CA<sub>warm</sub>, while accounting for the liquid water path and local environment. We estimate the ERFaci<sub>warm</sub>&nbsp;to be&nbsp;<span tabindex="0" data-mathml="&lt;math xmlns=&quot;http://www.w3.org/1998/Math/MathML&quot; id=&quot;M4&quot; display=&quot;inline&quot; overflow=&quot;scroll&quot; dspmath=&quot;mathml&quot;&gt;&lt;mrow&gt;&lt;mo&gt;-&lt;/mo&gt;&lt;mn mathvariant=&quot;normal&quot;&gt;0.32&lt;/mn&gt;&lt;mo&gt;&amp;#xB1;&lt;/mo&gt;&lt;mn mathvariant=&quot;normal&quot;&gt;0.16&lt;/mn&gt;&lt;/mrow&gt;&lt;/math&gt;">&minus;0.32&plusmn;0.16</span>&thinsp;Wm<sup>&minus;2</sup>. The RFaci<sub>warm</sub>&nbsp;dominates the ERFaci<sub>warm</sub>&nbsp;contributing 80&thinsp;% (<span tabindex="0" data-mathml="&lt;math xmlns=&quot;http://www.w3.org/1998/Math/MathML&quot; id=&quot;M8&quot; display=&quot;inline&quot; overflow=&quot;scroll&quot; dspmath=&quot;mathml&quot;&gt;&lt;mrow&gt;&lt;mo&gt;-&lt;/mo&gt;&lt;mn mathvariant=&quot;normal&quot;&gt;0.21&lt;/mn&gt;&lt;mo&gt;&amp;#xB1;&lt;/mo&gt;&lt;mn mathvariant=&quot;normal&quot;&gt;0.15&lt;/mn&gt;&lt;/mrow&gt;&lt;/math&gt;">&minus;0.21&plusmn;0.15</span>&thinsp;Wm<sup>&minus;2</sup>), while the CA<sub>warm</sub>&nbsp;enhances this cooling by 20&thinsp;% (<span tabindex="0" data-mathml="&lt;math xmlns=&quot;http://www.w3.org/1998/Math/MathML&quot; id=&quot;M11&quot; display=&quot;inline&quot; overflow=&quot;scroll&quot; dspmath=&quot;mathml&quot;&gt;&lt;mrow&gt;&lt;mo&gt;-&lt;/mo&gt;&lt;mn mathvariant=&quot;normal&quot;&gt;0.05&lt;/mn&gt;&lt;mo&gt;&amp;#xB1;&lt;/mo&gt;&lt;mn mathvariant=&quot;normal&quot;&gt;0.03&lt;/mn&gt;&lt;/mrow&gt;&lt;/math&gt;">&minus;0.05&plusmn;0.03</span>&thinsp;Wm<sup>&minus;2</sup>). Both the RFaci<sub>warm</sub>&nbsp;and CA<sub>warm</sub>&nbsp;vary in magnitude and sign regionally and can lead to opposite, negating effects under certain environmental conditions. Without considering the two terms separately and without constraining cloud&ndash;environment interactions, weak regional ERFaci<sub>warm</sub>&nbsp;signals may be erroneously attributed to a damped susceptibility to aerosol.</p>