Spray printing and optimization of anodes and cathodes for high performance Li-Ion batteries
A spray printing manufacturing approach to lithium-ion batteries was investigated with a focus on minimizing inactive fractions and maximizing energy and power densities of printable electrodes. Using a lithium titanate based anode initially and comparing with conventional electrodes, the effects of...
| Main Authors: | , , , |
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| Format: | Journal article |
| Language: | English |
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Elsevier
2018
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| _version_ | 1797084599676829696 |
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| author | Lee, S Huang, C Johnston, C Grant, P |
| author_facet | Lee, S Huang, C Johnston, C Grant, P |
| author_sort | Lee, S |
| collection | OXFORD |
| description | A spray printing manufacturing approach to lithium-ion batteries was investigated with a focus on minimizing inactive fractions and maximizing energy and power densities of printable electrodes. Using a lithium titanate based anode initially and comparing with conventional electrodes, the effects of conductivity enhancer and binder fractions, post-calendaring effects, different electrode manufacturing methods, conductivity enhancer types and electrode thicknesses were explored, and optimum electrode structures were identified. These insights were then applied to a lithium iron phosphate based cathode, and full spray printed lithium titanate/lithium iron phosphate cell configurations were investigated. Notably, the full-cell battery with a 1:1 capacity ratio of lithium titanate to lithium iron phosphate had a stable specific energy density of ∼300 Wh/kg and a power density of ∼2500 W/kg, showing the promise of layer-by-layer spray printing to realize fully the intrinsic properties of electrode materials in lithium-ion battery cells. |
| first_indexed | 2024-03-07T01:57:19Z |
| format | Journal article |
| id | oxford-uuid:9c2651cf-4e37-47cb-b454-a13c5686d1ec |
| institution | University of Oxford |
| language | English |
| last_indexed | 2024-03-07T01:57:19Z |
| publishDate | 2018 |
| publisher | Elsevier |
| record_format | dspace |
| spelling | oxford-uuid:9c2651cf-4e37-47cb-b454-a13c5686d1ec2022-03-27T00:34:03ZSpray printing and optimization of anodes and cathodes for high performance Li-Ion batteriesJournal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:9c2651cf-4e37-47cb-b454-a13c5686d1ecEnglishSymplectic Elements at OxfordElsevier2018Lee, SHuang, CJohnston, CGrant, PA spray printing manufacturing approach to lithium-ion batteries was investigated with a focus on minimizing inactive fractions and maximizing energy and power densities of printable electrodes. Using a lithium titanate based anode initially and comparing with conventional electrodes, the effects of conductivity enhancer and binder fractions, post-calendaring effects, different electrode manufacturing methods, conductivity enhancer types and electrode thicknesses were explored, and optimum electrode structures were identified. These insights were then applied to a lithium iron phosphate based cathode, and full spray printed lithium titanate/lithium iron phosphate cell configurations were investigated. Notably, the full-cell battery with a 1:1 capacity ratio of lithium titanate to lithium iron phosphate had a stable specific energy density of ∼300 Wh/kg and a power density of ∼2500 W/kg, showing the promise of layer-by-layer spray printing to realize fully the intrinsic properties of electrode materials in lithium-ion battery cells. |
| spellingShingle | Lee, S Huang, C Johnston, C Grant, P Spray printing and optimization of anodes and cathodes for high performance Li-Ion batteries |
| title | Spray printing and optimization of anodes and cathodes for high performance Li-Ion batteries |
| title_full | Spray printing and optimization of anodes and cathodes for high performance Li-Ion batteries |
| title_fullStr | Spray printing and optimization of anodes and cathodes for high performance Li-Ion batteries |
| title_full_unstemmed | Spray printing and optimization of anodes and cathodes for high performance Li-Ion batteries |
| title_short | Spray printing and optimization of anodes and cathodes for high performance Li-Ion batteries |
| title_sort | spray printing and optimization of anodes and cathodes for high performance li ion batteries |
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