Observation of structural anisotropy and the onset of liquidlike motion during the nonthermal melting of InSb.

The melting dynamics of laser excited InSb have been studied with femtosecond x-ray diffraction. These measurements observe the delayed onset of diffusive atomic motion, signaling the appearance of liquidlike dynamics. They also demonstrate that the root-mean-squared displacement in the [111] direct...

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Main Authors: Gaffney, K, Lindenberg, A, Larsson, J, Sokolowski-Tinten, K, Blome, C, Synnergren, O, Sheppard, J, Caleman, C, MacPhee, A, Weinstein, D, Lowney, D, Allison, T, Matthews, T, Falcone, R, Cavalieri, A, Fritz, D, Lee, S, Bucksbaum, P, Reis, D, Rudati, J, Macrander, A, Fuoss, P, Kao, C, Siddons, D, Pahl, R
Format: Journal article
Language:English
Published: 2005
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author Gaffney, K
Lindenberg, A
Larsson, J
Sokolowski-Tinten, K
Blome, C
Synnergren, O
Sheppard, J
Caleman, C
MacPhee, A
Weinstein, D
Lowney, D
Allison, T
Matthews, T
Falcone, R
Cavalieri, A
Fritz, D
Lee, S
Bucksbaum, P
Reis, D
Rudati, J
Macrander, A
Fuoss, P
Kao, C
Siddons, D
Pahl, R
author_facet Gaffney, K
Lindenberg, A
Larsson, J
Sokolowski-Tinten, K
Blome, C
Synnergren, O
Sheppard, J
Caleman, C
MacPhee, A
Weinstein, D
Lowney, D
Allison, T
Matthews, T
Falcone, R
Cavalieri, A
Fritz, D
Lee, S
Bucksbaum, P
Reis, D
Rudati, J
Macrander, A
Fuoss, P
Kao, C
Siddons, D
Pahl, R
author_sort Gaffney, K
collection OXFORD
description The melting dynamics of laser excited InSb have been studied with femtosecond x-ray diffraction. These measurements observe the delayed onset of diffusive atomic motion, signaling the appearance of liquidlike dynamics. They also demonstrate that the root-mean-squared displacement in the [111] direction increases faster than in the [110] direction after the first 500 fs. This structural anisotropy indicates that the initially generated fluid differs significantly from the equilibrium liquid.
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spelling oxford-uuid:9c83a7f9-dfd2-4702-bf02-e2cd060f91dd2022-03-27T00:36:34ZObservation of structural anisotropy and the onset of liquidlike motion during the nonthermal melting of InSb.Journal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:9c83a7f9-dfd2-4702-bf02-e2cd060f91ddEnglishSymplectic Elements at Oxford2005Gaffney, KLindenberg, ALarsson, JSokolowski-Tinten, KBlome, CSynnergren, OSheppard, JCaleman, CMacPhee, AWeinstein, DLowney, DAllison, TMatthews, TFalcone, RCavalieri, AFritz, DLee, SBucksbaum, PReis, DRudati, JMacrander, AFuoss, PKao, CSiddons, DPahl, RThe melting dynamics of laser excited InSb have been studied with femtosecond x-ray diffraction. These measurements observe the delayed onset of diffusive atomic motion, signaling the appearance of liquidlike dynamics. They also demonstrate that the root-mean-squared displacement in the [111] direction increases faster than in the [110] direction after the first 500 fs. This structural anisotropy indicates that the initially generated fluid differs significantly from the equilibrium liquid.
spellingShingle Gaffney, K
Lindenberg, A
Larsson, J
Sokolowski-Tinten, K
Blome, C
Synnergren, O
Sheppard, J
Caleman, C
MacPhee, A
Weinstein, D
Lowney, D
Allison, T
Matthews, T
Falcone, R
Cavalieri, A
Fritz, D
Lee, S
Bucksbaum, P
Reis, D
Rudati, J
Macrander, A
Fuoss, P
Kao, C
Siddons, D
Pahl, R
Observation of structural anisotropy and the onset of liquidlike motion during the nonthermal melting of InSb.
title Observation of structural anisotropy and the onset of liquidlike motion during the nonthermal melting of InSb.
title_full Observation of structural anisotropy and the onset of liquidlike motion during the nonthermal melting of InSb.
title_fullStr Observation of structural anisotropy and the onset of liquidlike motion during the nonthermal melting of InSb.
title_full_unstemmed Observation of structural anisotropy and the onset of liquidlike motion during the nonthermal melting of InSb.
title_short Observation of structural anisotropy and the onset of liquidlike motion during the nonthermal melting of InSb.
title_sort observation of structural anisotropy and the onset of liquidlike motion during the nonthermal melting of insb
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