Evolution of strain localization in glassy polymers: A numerical study

An explicit numerical implementation is described, for a constitutive model of glassy polymers, previously proposed and validated. Then it is exploited within a Finite Element continuum model, to simulate spontaneous strain localization (necking) occurring during extension of a prismatic bar of a ty...

Full description

Bibliographic Details
Main Authors: Li, H, Buckley, C
Format: Journal article
Language:English
Published: 2009
_version_ 1797085375269699584
author Li, H
Buckley, C
author_facet Li, H
Buckley, C
author_sort Li, H
collection OXFORD
description An explicit numerical implementation is described, for a constitutive model of glassy polymers, previously proposed and validated. Then it is exploited within a Finite Element continuum model, to simulate spontaneous strain localization (necking) occurring during extension of a prismatic bar of a typical glassy polymer. Material parameters for atactic polystyrene are employed. The material model is physically based and highly non-linearly viscoelastic. Three of its principal features are critical in simulations of strain localization: rate-dependence of plastic flow stress; strain-induced structural rejuvenation, represented by increase of Tool's fictive temperature and leading to pronounced post-yield strain softening; and molecular alignment during extension, giving rise to strain-hardening. In all simulations there is a peak in nominal stress, satisfying the condition for localization to occur. Nevertheless, the simulations show that the process of strain localization varies considerably, depending on details of the extension sequence and on assumed values for certain material parameters. A characteristic feature observed is that strain localization in such a material occurs in two stages. There is an initial spurt associated with strain-softening, followed by a slower growth of localization that eventually subsides, ultimately giving way to uniform extension of the neck. But the details of evolution of the strain distribution vary greatly. The rapidity and severity of localization are increased by decreased temperature, increased strain-rate or greater structural rejuvenation. A simple one-dimensional stability analysis is successful in explaining the results. © 2008 Elsevier Ltd. All rights reserved.
first_indexed 2024-03-07T02:08:05Z
format Journal article
id oxford-uuid:9fab3f1a-f1d6-42ee-aa89-cf7c4f1db3ca
institution University of Oxford
language English
last_indexed 2024-03-07T02:08:05Z
publishDate 2009
record_format dspace
spelling oxford-uuid:9fab3f1a-f1d6-42ee-aa89-cf7c4f1db3ca2022-03-27T00:59:42ZEvolution of strain localization in glassy polymers: A numerical studyJournal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:9fab3f1a-f1d6-42ee-aa89-cf7c4f1db3caEnglishSymplectic Elements at Oxford2009Li, HBuckley, CAn explicit numerical implementation is described, for a constitutive model of glassy polymers, previously proposed and validated. Then it is exploited within a Finite Element continuum model, to simulate spontaneous strain localization (necking) occurring during extension of a prismatic bar of a typical glassy polymer. Material parameters for atactic polystyrene are employed. The material model is physically based and highly non-linearly viscoelastic. Three of its principal features are critical in simulations of strain localization: rate-dependence of plastic flow stress; strain-induced structural rejuvenation, represented by increase of Tool's fictive temperature and leading to pronounced post-yield strain softening; and molecular alignment during extension, giving rise to strain-hardening. In all simulations there is a peak in nominal stress, satisfying the condition for localization to occur. Nevertheless, the simulations show that the process of strain localization varies considerably, depending on details of the extension sequence and on assumed values for certain material parameters. A characteristic feature observed is that strain localization in such a material occurs in two stages. There is an initial spurt associated with strain-softening, followed by a slower growth of localization that eventually subsides, ultimately giving way to uniform extension of the neck. But the details of evolution of the strain distribution vary greatly. The rapidity and severity of localization are increased by decreased temperature, increased strain-rate or greater structural rejuvenation. A simple one-dimensional stability analysis is successful in explaining the results. © 2008 Elsevier Ltd. All rights reserved.
spellingShingle Li, H
Buckley, C
Evolution of strain localization in glassy polymers: A numerical study
title Evolution of strain localization in glassy polymers: A numerical study
title_full Evolution of strain localization in glassy polymers: A numerical study
title_fullStr Evolution of strain localization in glassy polymers: A numerical study
title_full_unstemmed Evolution of strain localization in glassy polymers: A numerical study
title_short Evolution of strain localization in glassy polymers: A numerical study
title_sort evolution of strain localization in glassy polymers a numerical study
work_keys_str_mv AT lih evolutionofstrainlocalizationinglassypolymersanumericalstudy
AT buckleyc evolutionofstrainlocalizationinglassypolymersanumericalstudy