Novel stacking design of a flexible thin-film thermoelectric generator with a metal-insulator-semiconductor architecture

A stacked thermoelectric generator on a flexible polymer sheet is investigated that can utilize a low-cost high throughput roll-to-roll process, employing a metal–insulator–semiconductor structure of <100 nm thick Cu and bismuth telluride films with a ≈1 µm thick acrylate insulating coating. Ther...

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Main Authors: Tao, X, Hao, B, Assender, H
Format: Journal article
Language:English
Published: Wiley 2021
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author Tao, X
Hao, B
Assender, H
author_facet Tao, X
Hao, B
Assender, H
author_sort Tao, X
collection OXFORD
description A stacked thermoelectric generator on a flexible polymer sheet is investigated that can utilize a low-cost high throughput roll-to-roll process, employing a metal–insulator–semiconductor structure of <100 nm thick Cu and bismuth telluride films with a ≈1 µm thick acrylate insulating coating. Thermoelectric strips can be stacked and connected in the out-of-plane direction, which significantly decreases the size required in the substrate plane and also gives rise to the opportunity for greatly extending power output by stacking thousands of layers. A smooth surface of stacked layers is confirmed due to the nature of the acrylate layer. Room-temperature sputtering can produce good quality/crystalline films, indicated by X-ray diffraction and transmission electron microscope. Both experimental and simulation results observe a small temperature gradient across the stack from the bottom heat source to the top free surface. A stacked thermoelectric generator shows comparable performance to an in-plane device, and most notably, the stacked architecture allows a higher power output without increasing the dimension of the device in the substrate plane, while the thickness is increased within only a µm range. Cyclic buckling fatigue tests suggest that the performance of stacked functional strips can be protected under deformation within the acrylate matrix.
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spelling oxford-uuid:a0f66082-7d4a-483f-9f5d-938dd4dbdb9b2022-03-27T02:09:36ZNovel stacking design of a flexible thin-film thermoelectric generator with a metal-insulator-semiconductor architectureJournal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:a0f66082-7d4a-483f-9f5d-938dd4dbdb9bEnglishSymplectic ElementsWiley2021Tao, XHao, BAssender, HA stacked thermoelectric generator on a flexible polymer sheet is investigated that can utilize a low-cost high throughput roll-to-roll process, employing a metal–insulator–semiconductor structure of <100 nm thick Cu and bismuth telluride films with a ≈1 µm thick acrylate insulating coating. Thermoelectric strips can be stacked and connected in the out-of-plane direction, which significantly decreases the size required in the substrate plane and also gives rise to the opportunity for greatly extending power output by stacking thousands of layers. A smooth surface of stacked layers is confirmed due to the nature of the acrylate layer. Room-temperature sputtering can produce good quality/crystalline films, indicated by X-ray diffraction and transmission electron microscope. Both experimental and simulation results observe a small temperature gradient across the stack from the bottom heat source to the top free surface. A stacked thermoelectric generator shows comparable performance to an in-plane device, and most notably, the stacked architecture allows a higher power output without increasing the dimension of the device in the substrate plane, while the thickness is increased within only a µm range. Cyclic buckling fatigue tests suggest that the performance of stacked functional strips can be protected under deformation within the acrylate matrix.
spellingShingle Tao, X
Hao, B
Assender, H
Novel stacking design of a flexible thin-film thermoelectric generator with a metal-insulator-semiconductor architecture
title Novel stacking design of a flexible thin-film thermoelectric generator with a metal-insulator-semiconductor architecture
title_full Novel stacking design of a flexible thin-film thermoelectric generator with a metal-insulator-semiconductor architecture
title_fullStr Novel stacking design of a flexible thin-film thermoelectric generator with a metal-insulator-semiconductor architecture
title_full_unstemmed Novel stacking design of a flexible thin-film thermoelectric generator with a metal-insulator-semiconductor architecture
title_short Novel stacking design of a flexible thin-film thermoelectric generator with a metal-insulator-semiconductor architecture
title_sort novel stacking design of a flexible thin film thermoelectric generator with a metal insulator semiconductor architecture
work_keys_str_mv AT taox novelstackingdesignofaflexiblethinfilmthermoelectricgeneratorwithametalinsulatorsemiconductorarchitecture
AT haob novelstackingdesignofaflexiblethinfilmthermoelectricgeneratorwithametalinsulatorsemiconductorarchitecture
AT assenderh novelstackingdesignofaflexiblethinfilmthermoelectricgeneratorwithametalinsulatorsemiconductorarchitecture