Novel stacking design of a flexible thin-film thermoelectric generator with a metal-insulator-semiconductor architecture
A stacked thermoelectric generator on a flexible polymer sheet is investigated that can utilize a low-cost high throughput roll-to-roll process, employing a metal–insulator–semiconductor structure of <100 nm thick Cu and bismuth telluride films with a ≈1 µm thick acrylate insulating coating. Ther...
Main Authors: | , , |
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Format: | Journal article |
Language: | English |
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Wiley
2021
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author | Tao, X Hao, B Assender, H |
author_facet | Tao, X Hao, B Assender, H |
author_sort | Tao, X |
collection | OXFORD |
description | A stacked thermoelectric generator on a flexible polymer sheet is investigated that can utilize a low-cost high throughput roll-to-roll process, employing a metal–insulator–semiconductor structure of <100 nm thick Cu and bismuth telluride films with a ≈1 µm thick acrylate insulating coating. Thermoelectric strips can be stacked and connected in the out-of-plane direction, which significantly decreases the size required in the substrate plane and also gives rise to the opportunity for greatly extending power output by stacking thousands of layers. A smooth surface of stacked layers is confirmed due to the nature of the acrylate layer. Room-temperature sputtering can produce good quality/crystalline films, indicated by X-ray diffraction and transmission electron microscope. Both experimental and simulation results observe a small temperature gradient across the stack from the bottom heat source to the top free surface. A stacked thermoelectric generator shows comparable performance to an in-plane device, and most notably, the stacked architecture allows a higher power output without increasing the dimension of the device in the substrate plane, while the thickness is increased within only a µm range. Cyclic buckling fatigue tests suggest that the performance of stacked functional strips can be protected under deformation within the acrylate matrix.
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first_indexed | 2024-03-07T02:11:58Z |
format | Journal article |
id | oxford-uuid:a0f66082-7d4a-483f-9f5d-938dd4dbdb9b |
institution | University of Oxford |
language | English |
last_indexed | 2024-03-07T02:11:58Z |
publishDate | 2021 |
publisher | Wiley |
record_format | dspace |
spelling | oxford-uuid:a0f66082-7d4a-483f-9f5d-938dd4dbdb9b2022-03-27T02:09:36ZNovel stacking design of a flexible thin-film thermoelectric generator with a metal-insulator-semiconductor architectureJournal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:a0f66082-7d4a-483f-9f5d-938dd4dbdb9bEnglishSymplectic ElementsWiley2021Tao, XHao, BAssender, HA stacked thermoelectric generator on a flexible polymer sheet is investigated that can utilize a low-cost high throughput roll-to-roll process, employing a metal–insulator–semiconductor structure of <100 nm thick Cu and bismuth telluride films with a ≈1 µm thick acrylate insulating coating. Thermoelectric strips can be stacked and connected in the out-of-plane direction, which significantly decreases the size required in the substrate plane and also gives rise to the opportunity for greatly extending power output by stacking thousands of layers. A smooth surface of stacked layers is confirmed due to the nature of the acrylate layer. Room-temperature sputtering can produce good quality/crystalline films, indicated by X-ray diffraction and transmission electron microscope. Both experimental and simulation results observe a small temperature gradient across the stack from the bottom heat source to the top free surface. A stacked thermoelectric generator shows comparable performance to an in-plane device, and most notably, the stacked architecture allows a higher power output without increasing the dimension of the device in the substrate plane, while the thickness is increased within only a µm range. Cyclic buckling fatigue tests suggest that the performance of stacked functional strips can be protected under deformation within the acrylate matrix. |
spellingShingle | Tao, X Hao, B Assender, H Novel stacking design of a flexible thin-film thermoelectric generator with a metal-insulator-semiconductor architecture |
title | Novel stacking design of a flexible thin-film thermoelectric generator with a metal-insulator-semiconductor architecture |
title_full | Novel stacking design of a flexible thin-film thermoelectric generator with a metal-insulator-semiconductor architecture |
title_fullStr | Novel stacking design of a flexible thin-film thermoelectric generator with a metal-insulator-semiconductor architecture |
title_full_unstemmed | Novel stacking design of a flexible thin-film thermoelectric generator with a metal-insulator-semiconductor architecture |
title_short | Novel stacking design of a flexible thin-film thermoelectric generator with a metal-insulator-semiconductor architecture |
title_sort | novel stacking design of a flexible thin film thermoelectric generator with a metal insulator semiconductor architecture |
work_keys_str_mv | AT taox novelstackingdesignofaflexiblethinfilmthermoelectricgeneratorwithametalinsulatorsemiconductorarchitecture AT haob novelstackingdesignofaflexiblethinfilmthermoelectricgeneratorwithametalinsulatorsemiconductorarchitecture AT assenderh novelstackingdesignofaflexiblethinfilmthermoelectricgeneratorwithametalinsulatorsemiconductorarchitecture |