Driven spheres, ellipsoids and rods in explicitly modeled polymer solutions

Understanding the transport of driven nano- and micro-particles in complex fluids is of relevance for many biological and technological applications. Here we perform hydrodynamic multiparticle collision dynamics simulations of spherical and elongated particles driven through polymeric fluids contain...

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Main Authors: Zöttl, A, Yeomans, JM
Format: Journal article
Language:English
Published: IOP Publishing 2019
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author Zöttl, A
Yeomans, JM
author_facet Zöttl, A
Yeomans, JM
author_sort Zöttl, A
collection OXFORD
description Understanding the transport of driven nano- and micro-particles in complex fluids is of relevance for many biological and technological applications. Here we perform hydrodynamic multiparticle collision dynamics simulations of spherical and elongated particles driven through polymeric fluids containing different concentrations of polymers. We determine the mean particle velocities which are larger than expected from Stokes law for all particle shapes and polymer densities. Furthermore we measure the fluid flow fields and local polymer density and polymer conformation around the particles. We find that polymer-depleted regions close to the particles are responsible for an apparent tangential slip velocity which accounts for the measured flow fields and transport velocities. A simple two-layer fluid model gives a good match to the simulation results.
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spelling oxford-uuid:a1e7e363-645a-418a-93bb-0563eb30f70a2022-03-27T02:16:32ZDriven spheres, ellipsoids and rods in explicitly modeled polymer solutionsJournal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:a1e7e363-645a-418a-93bb-0563eb30f70aEnglishSymplectic Elements at OxfordIOP Publishing2019Zöttl, AYeomans, JMUnderstanding the transport of driven nano- and micro-particles in complex fluids is of relevance for many biological and technological applications. Here we perform hydrodynamic multiparticle collision dynamics simulations of spherical and elongated particles driven through polymeric fluids containing different concentrations of polymers. We determine the mean particle velocities which are larger than expected from Stokes law for all particle shapes and polymer densities. Furthermore we measure the fluid flow fields and local polymer density and polymer conformation around the particles. We find that polymer-depleted regions close to the particles are responsible for an apparent tangential slip velocity which accounts for the measured flow fields and transport velocities. A simple two-layer fluid model gives a good match to the simulation results.
spellingShingle Zöttl, A
Yeomans, JM
Driven spheres, ellipsoids and rods in explicitly modeled polymer solutions
title Driven spheres, ellipsoids and rods in explicitly modeled polymer solutions
title_full Driven spheres, ellipsoids and rods in explicitly modeled polymer solutions
title_fullStr Driven spheres, ellipsoids and rods in explicitly modeled polymer solutions
title_full_unstemmed Driven spheres, ellipsoids and rods in explicitly modeled polymer solutions
title_short Driven spheres, ellipsoids and rods in explicitly modeled polymer solutions
title_sort driven spheres ellipsoids and rods in explicitly modeled polymer solutions
work_keys_str_mv AT zottla drivenspheresellipsoidsandrodsinexplicitlymodeledpolymersolutions
AT yeomansjm drivenspheresellipsoidsandrodsinexplicitlymodeledpolymersolutions