Grain-boundary fluctuations in two-dimensional colloidal crystals.

We study grain-boundary fluctuations in two-dimensional colloidal crystals in real space and time using video microscopy. The experimentally obtained static and dynamic correlation functions are very well described by expressions obtained using capillary wave theory. This directly leads to values fo...

Full description

Bibliographic Details
Main Authors: Skinner, T, Aarts, D, Dullens, R
Format: Journal article
Language:English
Published: 2010
_version_ 1797087843893379072
author Skinner, T
Aarts, D
Dullens, R
author_facet Skinner, T
Aarts, D
Dullens, R
author_sort Skinner, T
collection OXFORD
description We study grain-boundary fluctuations in two-dimensional colloidal crystals in real space and time using video microscopy. The experimentally obtained static and dynamic correlation functions are very well described by expressions obtained using capillary wave theory. This directly leads to values for the interfacial stiffness and the interface mobility, the key parameters in curvature-driven grain-boundary migration. Furthermore, we show that the average grain-boundary position exhibits a one-dimensional random walk as recently suggested by computer simulations [Z. T. Trautt, M. Upmanyu, and A. Karma, Science 314, 632 (2006)]. The interface mobility determined from the mean-square displacement of the average grain-boundary position is in good agreement with values inferred from grain-boundary fluctuations.
first_indexed 2024-03-07T02:41:24Z
format Journal article
id oxford-uuid:aa9309a5-c5e2-475f-8fd3-7b6fc84d1e7c
institution University of Oxford
language English
last_indexed 2024-03-07T02:41:24Z
publishDate 2010
record_format dspace
spelling oxford-uuid:aa9309a5-c5e2-475f-8fd3-7b6fc84d1e7c2022-03-27T03:16:03ZGrain-boundary fluctuations in two-dimensional colloidal crystals.Journal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:aa9309a5-c5e2-475f-8fd3-7b6fc84d1e7cEnglishSymplectic Elements at Oxford2010Skinner, TAarts, DDullens, RWe study grain-boundary fluctuations in two-dimensional colloidal crystals in real space and time using video microscopy. The experimentally obtained static and dynamic correlation functions are very well described by expressions obtained using capillary wave theory. This directly leads to values for the interfacial stiffness and the interface mobility, the key parameters in curvature-driven grain-boundary migration. Furthermore, we show that the average grain-boundary position exhibits a one-dimensional random walk as recently suggested by computer simulations [Z. T. Trautt, M. Upmanyu, and A. Karma, Science 314, 632 (2006)]. The interface mobility determined from the mean-square displacement of the average grain-boundary position is in good agreement with values inferred from grain-boundary fluctuations.
spellingShingle Skinner, T
Aarts, D
Dullens, R
Grain-boundary fluctuations in two-dimensional colloidal crystals.
title Grain-boundary fluctuations in two-dimensional colloidal crystals.
title_full Grain-boundary fluctuations in two-dimensional colloidal crystals.
title_fullStr Grain-boundary fluctuations in two-dimensional colloidal crystals.
title_full_unstemmed Grain-boundary fluctuations in two-dimensional colloidal crystals.
title_short Grain-boundary fluctuations in two-dimensional colloidal crystals.
title_sort grain boundary fluctuations in two dimensional colloidal crystals
work_keys_str_mv AT skinnert grainboundaryfluctuationsintwodimensionalcolloidalcrystals
AT aartsd grainboundaryfluctuationsintwodimensionalcolloidalcrystals
AT dullensr grainboundaryfluctuationsintwodimensionalcolloidalcrystals