Electron spin coherence and electron nuclear double resonance of Bi donors in natural Si.

Donors in silicon hold considerable promise for emerging quantum technologies, due to their uniquely long electron spin coherence times. Bismuth donors in silicon differ from more widely studied group V donors, such as phosphorous, in several significant respects: They have the strongest binding ene...

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Main Authors: George, R, Witzel, W, Riemann, H, Abrosimov, N, Nötzel, N, Thewalt, M, Morton, J
Format: Journal article
Jezik:English
Izdano: 2010
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author George, R
Witzel, W
Riemann, H
Abrosimov, N
Nötzel, N
Thewalt, M
Morton, J
author_facet George, R
Witzel, W
Riemann, H
Abrosimov, N
Nötzel, N
Thewalt, M
Morton, J
author_sort George, R
collection OXFORD
description Donors in silicon hold considerable promise for emerging quantum technologies, due to their uniquely long electron spin coherence times. Bismuth donors in silicon differ from more widely studied group V donors, such as phosphorous, in several significant respects: They have the strongest binding energy (70.98 meV), a large nuclear spin (I=9/2), and a strong hyperfine coupling constant (A=1475.4  MHz). These larger energy scales allow us to perform a detailed test of theoretical models describing the spectral diffusion mechanism that is known to govern the electron spin decoherence of P donors in natural silicon. We report the electron-nuclear double resonance spectra of the Bi donor, across the range 200 MHz to 1.4 GHz, and confirm that coherence transfer is possible between electron and nuclear spin degrees of freedom at these higher frequencies.
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spelling oxford-uuid:abd9775d-b095-4b46-a5c6-531ea5ea3b512022-03-27T03:24:44ZElectron spin coherence and electron nuclear double resonance of Bi donors in natural Si.Journal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:abd9775d-b095-4b46-a5c6-531ea5ea3b51EnglishSymplectic Elements at Oxford2010George, RWitzel, WRiemann, HAbrosimov, NNötzel, NThewalt, MMorton, JDonors in silicon hold considerable promise for emerging quantum technologies, due to their uniquely long electron spin coherence times. Bismuth donors in silicon differ from more widely studied group V donors, such as phosphorous, in several significant respects: They have the strongest binding energy (70.98 meV), a large nuclear spin (I=9/2), and a strong hyperfine coupling constant (A=1475.4  MHz). These larger energy scales allow us to perform a detailed test of theoretical models describing the spectral diffusion mechanism that is known to govern the electron spin decoherence of P donors in natural silicon. We report the electron-nuclear double resonance spectra of the Bi donor, across the range 200 MHz to 1.4 GHz, and confirm that coherence transfer is possible between electron and nuclear spin degrees of freedom at these higher frequencies.
spellingShingle George, R
Witzel, W
Riemann, H
Abrosimov, N
Nötzel, N
Thewalt, M
Morton, J
Electron spin coherence and electron nuclear double resonance of Bi donors in natural Si.
title Electron spin coherence and electron nuclear double resonance of Bi donors in natural Si.
title_full Electron spin coherence and electron nuclear double resonance of Bi donors in natural Si.
title_fullStr Electron spin coherence and electron nuclear double resonance of Bi donors in natural Si.
title_full_unstemmed Electron spin coherence and electron nuclear double resonance of Bi donors in natural Si.
title_short Electron spin coherence and electron nuclear double resonance of Bi donors in natural Si.
title_sort electron spin coherence and electron nuclear double resonance of bi donors in natural si
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AT abrosimovn electronspincoherenceandelectronnucleardoubleresonanceofbidonorsinnaturalsi
AT notzeln electronspincoherenceandelectronnucleardoubleresonanceofbidonorsinnaturalsi
AT thewaltm electronspincoherenceandelectronnucleardoubleresonanceofbidonorsinnaturalsi
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