Ultrafast optical excitation of a persistent surface-state population in the topological insulator Bi2Se3.
Using femtosecond time- and angle-resolved photoemission spectroscopy, we investigated the nonequilibrium dynamics of the topological insulator Bi2Se3. We studied p-type Bi2Se3, in which the metallic Dirac surface state and bulk conduction bands are unoccupied. Optical excitation leads to a metastab...
Main Authors: | , , , , , , |
---|---|
Format: | Journal article |
Language: | English |
Published: |
2012
|
_version_ | 1797088253200826368 |
---|---|
author | Sobota, J Yang, S Analytis, J Chen, Y Fisher, I Kirchmann, P Shen, Z |
author_facet | Sobota, J Yang, S Analytis, J Chen, Y Fisher, I Kirchmann, P Shen, Z |
author_sort | Sobota, J |
collection | OXFORD |
description | Using femtosecond time- and angle-resolved photoemission spectroscopy, we investigated the nonequilibrium dynamics of the topological insulator Bi2Se3. We studied p-type Bi2Se3, in which the metallic Dirac surface state and bulk conduction bands are unoccupied. Optical excitation leads to a metastable population at the bulk conduction band edge, which feeds a nonequilibrium population of the surface state persisting for >10 ps. This unusually long-lived population of a metallic Dirac surface state with spin texture may present a channel in which to drive transient spin-polarized currents. |
first_indexed | 2024-03-07T02:47:22Z |
format | Journal article |
id | oxford-uuid:ac7bc455-d5e4-4a62-ac0f-ba4d65c2c1fc |
institution | University of Oxford |
language | English |
last_indexed | 2024-03-07T02:47:22Z |
publishDate | 2012 |
record_format | dspace |
spelling | oxford-uuid:ac7bc455-d5e4-4a62-ac0f-ba4d65c2c1fc2022-03-27T03:29:20ZUltrafast optical excitation of a persistent surface-state population in the topological insulator Bi2Se3.Journal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:ac7bc455-d5e4-4a62-ac0f-ba4d65c2c1fcEnglishSymplectic Elements at Oxford2012Sobota, JYang, SAnalytis, JChen, YFisher, IKirchmann, PShen, ZUsing femtosecond time- and angle-resolved photoemission spectroscopy, we investigated the nonequilibrium dynamics of the topological insulator Bi2Se3. We studied p-type Bi2Se3, in which the metallic Dirac surface state and bulk conduction bands are unoccupied. Optical excitation leads to a metastable population at the bulk conduction band edge, which feeds a nonequilibrium population of the surface state persisting for >10 ps. This unusually long-lived population of a metallic Dirac surface state with spin texture may present a channel in which to drive transient spin-polarized currents. |
spellingShingle | Sobota, J Yang, S Analytis, J Chen, Y Fisher, I Kirchmann, P Shen, Z Ultrafast optical excitation of a persistent surface-state population in the topological insulator Bi2Se3. |
title | Ultrafast optical excitation of a persistent surface-state population in the topological insulator Bi2Se3. |
title_full | Ultrafast optical excitation of a persistent surface-state population in the topological insulator Bi2Se3. |
title_fullStr | Ultrafast optical excitation of a persistent surface-state population in the topological insulator Bi2Se3. |
title_full_unstemmed | Ultrafast optical excitation of a persistent surface-state population in the topological insulator Bi2Se3. |
title_short | Ultrafast optical excitation of a persistent surface-state population in the topological insulator Bi2Se3. |
title_sort | ultrafast optical excitation of a persistent surface state population in the topological insulator bi2se3 |
work_keys_str_mv | AT sobotaj ultrafastopticalexcitationofapersistentsurfacestatepopulationinthetopologicalinsulatorbi2se3 AT yangs ultrafastopticalexcitationofapersistentsurfacestatepopulationinthetopologicalinsulatorbi2se3 AT analytisj ultrafastopticalexcitationofapersistentsurfacestatepopulationinthetopologicalinsulatorbi2se3 AT cheny ultrafastopticalexcitationofapersistentsurfacestatepopulationinthetopologicalinsulatorbi2se3 AT fisheri ultrafastopticalexcitationofapersistentsurfacestatepopulationinthetopologicalinsulatorbi2se3 AT kirchmannp ultrafastopticalexcitationofapersistentsurfacestatepopulationinthetopologicalinsulatorbi2se3 AT shenz ultrafastopticalexcitationofapersistentsurfacestatepopulationinthetopologicalinsulatorbi2se3 |