Glaciation of liquid clouds, snowfall and reduced cloud cover at industrial aerosol hot spots

The ability of anthropogenic aerosols to freeze supercooled cloud droplets remains debated. In this work, we present observational evidence for the glaciation of supercooled liquid-water clouds at industrial aerosol hot spots at temperatures between −10° and −24°C. Compared with the nearby liquid-wa...

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Main Authors: Toll, V, Rahu, J, Keernik, H, Trofimov, H, Voormansik, T, Manshausen, P, Hung, E, Michelson, D, Christensen, M, Post, P, Junninen, H, Murray, BJ, Lohmann, U, Watson-Parris, D, Stier, P, Donaldson, N, Storelvmo, T, Kulmala, M, Bellouin, N
Format: Journal article
Language:English
Published: American Association for the Advancement of Science 2024
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author Toll, V
Rahu, J
Keernik, H
Trofimov, H
Voormansik, T
Manshausen, P
Hung, E
Michelson, D
Christensen, M
Post, P
Junninen, H
Murray, BJ
Lohmann, U
Watson-Parris, D
Stier, P
Donaldson, N
Storelvmo, T
Kulmala, M
Bellouin, N
author_facet Toll, V
Rahu, J
Keernik, H
Trofimov, H
Voormansik, T
Manshausen, P
Hung, E
Michelson, D
Christensen, M
Post, P
Junninen, H
Murray, BJ
Lohmann, U
Watson-Parris, D
Stier, P
Donaldson, N
Storelvmo, T
Kulmala, M
Bellouin, N
author_sort Toll, V
collection OXFORD
description The ability of anthropogenic aerosols to freeze supercooled cloud droplets remains debated. In this work, we present observational evidence for the glaciation of supercooled liquid-water clouds at industrial aerosol hot spots at temperatures between −10° and −24°C. Compared with the nearby liquid-water clouds, shortwave reflectance was reduced by 14% and longwave radiance was increased by 4% in the glaciation-affected regions. There was an 8% reduction in cloud cover and an 18% reduction in cloud optical thickness. Additionally, daily glaciation-induced snowfall accumulations reached 15 millimeters. Glaciation events downwind of industrial aerosol hot spots indicate that anthropogenic aerosols likely serve as ice-nucleating particles. However, rare glaciation events downwind of nuclear power plants indicate that factors other than aerosol emissions may also play a role in the observed glaciation events.
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spelling oxford-uuid:acb3b94a-d418-408b-b127-e05d74cc7b5f2024-11-27T13:11:17ZGlaciation of liquid clouds, snowfall and reduced cloud cover at industrial aerosol hot spotsJournal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:acb3b94a-d418-408b-b127-e05d74cc7b5fEnglishSymplectic ElementsAmerican Association for the Advancement of Science2024Toll, VRahu, JKeernik, HTrofimov, HVoormansik, TManshausen, PHung, EMichelson, DChristensen, MPost, PJunninen, HMurray, BJLohmann, UWatson-Parris, DStier, PDonaldson, NStorelvmo, TKulmala, MBellouin, NThe ability of anthropogenic aerosols to freeze supercooled cloud droplets remains debated. In this work, we present observational evidence for the glaciation of supercooled liquid-water clouds at industrial aerosol hot spots at temperatures between −10° and −24°C. Compared with the nearby liquid-water clouds, shortwave reflectance was reduced by 14% and longwave radiance was increased by 4% in the glaciation-affected regions. There was an 8% reduction in cloud cover and an 18% reduction in cloud optical thickness. Additionally, daily glaciation-induced snowfall accumulations reached 15 millimeters. Glaciation events downwind of industrial aerosol hot spots indicate that anthropogenic aerosols likely serve as ice-nucleating particles. However, rare glaciation events downwind of nuclear power plants indicate that factors other than aerosol emissions may also play a role in the observed glaciation events.
spellingShingle Toll, V
Rahu, J
Keernik, H
Trofimov, H
Voormansik, T
Manshausen, P
Hung, E
Michelson, D
Christensen, M
Post, P
Junninen, H
Murray, BJ
Lohmann, U
Watson-Parris, D
Stier, P
Donaldson, N
Storelvmo, T
Kulmala, M
Bellouin, N
Glaciation of liquid clouds, snowfall and reduced cloud cover at industrial aerosol hot spots
title Glaciation of liquid clouds, snowfall and reduced cloud cover at industrial aerosol hot spots
title_full Glaciation of liquid clouds, snowfall and reduced cloud cover at industrial aerosol hot spots
title_fullStr Glaciation of liquid clouds, snowfall and reduced cloud cover at industrial aerosol hot spots
title_full_unstemmed Glaciation of liquid clouds, snowfall and reduced cloud cover at industrial aerosol hot spots
title_short Glaciation of liquid clouds, snowfall and reduced cloud cover at industrial aerosol hot spots
title_sort glaciation of liquid clouds snowfall and reduced cloud cover at industrial aerosol hot spots
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