Comparing neutron and helium ion irradiation damage of REBa2Cu3O7−δ coated conductor using X-ray absorption spectroscopy

Understanding the effects of high energy neutron damage on REBa2Cu3O$_{7-\delta}$ (REBCO) coated conductor is of vital importance for the design of the magnetic confinement systems for compact nuclear fusion power plants. However, neutron irradiation campaigns can only be carried out in a few facili...

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Main Authors: Adams, K, Iliffe, W, Nicholls, R, He, G, Diaz-Moreno, S, Mosselmans, F, Fischer, D, Eisterer, M, Grovenor, C, Speller, SC
Format: Journal article
Language:English
Published: IOP Publishing 2023
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author Adams, K
Iliffe, W
Nicholls, R
He, G
Diaz-Moreno, S
Mosselmans, F
Fischer, D
Eisterer, M
Grovenor, C
Speller, SC
author_facet Adams, K
Iliffe, W
Nicholls, R
He, G
Diaz-Moreno, S
Mosselmans, F
Fischer, D
Eisterer, M
Grovenor, C
Speller, SC
author_sort Adams, K
collection OXFORD
description Understanding the effects of high energy neutron damage on REBa2Cu3O$_{7-\delta}$ (REBCO) coated conductor is of vital importance for the design of the magnetic confinement systems for compact nuclear fusion power plants. However, neutron irradiation campaigns can only be carried out in a few facilities, and the experiments are very slow and expensive partly because the samples become radioactive. Ion irradiation provides an easily accessible alternative route to studying the effects of radiation on high temperature superconductors, which not only increases the volume of technical data that can be obtained but also enables more complex experiments such as in situ cryogenic irradiation. The question is, does ion damage offer a good proxy for neutrons? Here we use high energy resolution fluorescence detected x-ray absorption spectroscopy to probe the effects of fast neutron irradiation on the local environment around the copper ions in the REBCO layer of coated conductor tapes. We find that the spectral changes are similar to those induced by helium ion irradiation, suggesting that both projectiles produce the same types of structural defect in the REBCO lattice, although there is some evidence of an additional type of defect present in the sample heavily damaged by He+ ion irradiation. It is also shown that the linear degradation of superconducting transition temperature (Tc) of coated conductors with the calculated number of displacements per atom occurs at the same rate for neutrons and helium ions. Together these results provide new evidence suggesting that helium ions can emulate neutron point defect damage in REBCO high temperature superconductor reasonably well, increasing confidence that helium ions could be used as a useful proxy for neutrons in future experiments.
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spelling oxford-uuid:baef5a4b-5682-455e-8756-6ca84fe74af72023-11-09T07:20:49ZComparing neutron and helium ion irradiation damage of REBa2Cu3O7−δ coated conductor using X-ray absorption spectroscopyJournal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:baef5a4b-5682-455e-8756-6ca84fe74af7EnglishSymplectic ElementsIOP Publishing2023Adams, KIliffe, WNicholls, RHe, GDiaz-Moreno, SMosselmans, FFischer, DEisterer, MGrovenor, CSpeller, SCUnderstanding the effects of high energy neutron damage on REBa2Cu3O$_{7-\delta}$ (REBCO) coated conductor is of vital importance for the design of the magnetic confinement systems for compact nuclear fusion power plants. However, neutron irradiation campaigns can only be carried out in a few facilities, and the experiments are very slow and expensive partly because the samples become radioactive. Ion irradiation provides an easily accessible alternative route to studying the effects of radiation on high temperature superconductors, which not only increases the volume of technical data that can be obtained but also enables more complex experiments such as in situ cryogenic irradiation. The question is, does ion damage offer a good proxy for neutrons? Here we use high energy resolution fluorescence detected x-ray absorption spectroscopy to probe the effects of fast neutron irradiation on the local environment around the copper ions in the REBCO layer of coated conductor tapes. We find that the spectral changes are similar to those induced by helium ion irradiation, suggesting that both projectiles produce the same types of structural defect in the REBCO lattice, although there is some evidence of an additional type of defect present in the sample heavily damaged by He+ ion irradiation. It is also shown that the linear degradation of superconducting transition temperature (Tc) of coated conductors with the calculated number of displacements per atom occurs at the same rate for neutrons and helium ions. Together these results provide new evidence suggesting that helium ions can emulate neutron point defect damage in REBCO high temperature superconductor reasonably well, increasing confidence that helium ions could be used as a useful proxy for neutrons in future experiments.
spellingShingle Adams, K
Iliffe, W
Nicholls, R
He, G
Diaz-Moreno, S
Mosselmans, F
Fischer, D
Eisterer, M
Grovenor, C
Speller, SC
Comparing neutron and helium ion irradiation damage of REBa2Cu3O7−δ coated conductor using X-ray absorption spectroscopy
title Comparing neutron and helium ion irradiation damage of REBa2Cu3O7−δ coated conductor using X-ray absorption spectroscopy
title_full Comparing neutron and helium ion irradiation damage of REBa2Cu3O7−δ coated conductor using X-ray absorption spectroscopy
title_fullStr Comparing neutron and helium ion irradiation damage of REBa2Cu3O7−δ coated conductor using X-ray absorption spectroscopy
title_full_unstemmed Comparing neutron and helium ion irradiation damage of REBa2Cu3O7−δ coated conductor using X-ray absorption spectroscopy
title_short Comparing neutron and helium ion irradiation damage of REBa2Cu3O7−δ coated conductor using X-ray absorption spectroscopy
title_sort comparing neutron and helium ion irradiation damage of reba2cu3o7 δ coated conductor using x ray absorption spectroscopy
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