Ultrafast nonlinear spectroscopy of individual quantum dots: imaging and coherent coupling

We review our recent advances in four-wave mixing spectroscopy of individual semiconductor quantum dots using heterodyne spectral interferometry, a novel implementation of transient nonlinear spectroscopy allowing the study of the transient nonlinear polarization emitted from individual electronic t...

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Main Authors: Kasprzak, J, Patton, B, Langbein, W
Format: Conference item
Published: 2008
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author Kasprzak, J
Patton, B
Langbein, W
author_facet Kasprzak, J
Patton, B
Langbein, W
author_sort Kasprzak, J
collection OXFORD
description We review our recent advances in four-wave mixing spectroscopy of individual semiconductor quantum dots using heterodyne spectral interferometry, a novel implementation of transient nonlinear spectroscopy allowing the study of the transient nonlinear polarization emitted from individual electronic transitions in both amplitude and phase. We present experiments on individual excitonic transitions localized in monolayer islands of a GaAs/AlAs quantum well. The detection of amplitude and phase allows the implementation of a twodimensional femtosecond spectroscopy, in which mutual coherent coupling of single quantum dot states can be observed and quantified. By combining two-dimensional femtosecond spectroscopy with four-wave mixing mapping in the real space we found coherent coupling between spatially separated excitons by up to ~ 0.8 μm..
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spelling oxford-uuid:ced93252-9ce9-459b-af4a-65650c47ecc72022-03-27T07:38:24ZUltrafast nonlinear spectroscopy of individual quantum dots: imaging and coherent couplingConference itemhttp://purl.org/coar/resource_type/c_5794uuid:ced93252-9ce9-459b-af4a-65650c47ecc7Symplectic Elements at Oxford2008Kasprzak, JPatton, BLangbein, WWe review our recent advances in four-wave mixing spectroscopy of individual semiconductor quantum dots using heterodyne spectral interferometry, a novel implementation of transient nonlinear spectroscopy allowing the study of the transient nonlinear polarization emitted from individual electronic transitions in both amplitude and phase. We present experiments on individual excitonic transitions localized in monolayer islands of a GaAs/AlAs quantum well. The detection of amplitude and phase allows the implementation of a twodimensional femtosecond spectroscopy, in which mutual coherent coupling of single quantum dot states can be observed and quantified. By combining two-dimensional femtosecond spectroscopy with four-wave mixing mapping in the real space we found coherent coupling between spatially separated excitons by up to ~ 0.8 μm..
spellingShingle Kasprzak, J
Patton, B
Langbein, W
Ultrafast nonlinear spectroscopy of individual quantum dots: imaging and coherent coupling
title Ultrafast nonlinear spectroscopy of individual quantum dots: imaging and coherent coupling
title_full Ultrafast nonlinear spectroscopy of individual quantum dots: imaging and coherent coupling
title_fullStr Ultrafast nonlinear spectroscopy of individual quantum dots: imaging and coherent coupling
title_full_unstemmed Ultrafast nonlinear spectroscopy of individual quantum dots: imaging and coherent coupling
title_short Ultrafast nonlinear spectroscopy of individual quantum dots: imaging and coherent coupling
title_sort ultrafast nonlinear spectroscopy of individual quantum dots imaging and coherent coupling
work_keys_str_mv AT kasprzakj ultrafastnonlinearspectroscopyofindividualquantumdotsimagingandcoherentcoupling
AT pattonb ultrafastnonlinearspectroscopyofindividualquantumdotsimagingandcoherentcoupling
AT langbeinw ultrafastnonlinearspectroscopyofindividualquantumdotsimagingandcoherentcoupling