Quantum control of the tin-vacancy spin qubit in diamond

<p>Group-IV color centers in diamond are a promising light-matter interface for quantum networking devices. The negatively charged tin-vacancy center (<span tabindex="0">SnV</span>) is particularly interesting, as its large spin-orbit coupling offers strong protection aga...

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Bibliographic Details
Main Authors: Debroux, R, Michaels, CP, Purser, CM, Wan, N, Trusheim, ME, Martinez, JA, Parker, RA, Stramma, AM, Chen, KC, de Santis, L, Alexeev, EM, Ferrari, AC, Englund, D, Gangloff, DA, Atature, M
Format: Journal article
Language:English
Published: American Physical Society 2021
Description
Summary:<p>Group-IV color centers in diamond are a promising light-matter interface for quantum networking devices. The negatively charged tin-vacancy center (<span tabindex="0">SnV</span>) is particularly interesting, as its large spin-orbit coupling offers strong protection against phonon dephasing and robust cyclicity of its optical transitions toward spin-photon-entanglement schemes. Here, we demonstrate multiaxis coherent control of the&nbsp;<span tabindex="0">SnV</span>&nbsp;spin qubit via an all-optical stimulated Raman drive between the ground and excited states. We use coherent population trapping and optically driven electronic spin resonance to confirm coherent access to the qubit at 1.7&nbsp;K and obtain spin Rabi oscillations at a rate of&nbsp;<span tabindex="0">&Omega;/2&pi;=19.0(1)&thinsp;&thinsp;MHz</span>. All-optical Ramsey interferometry reveals a spin dephasing time of&nbsp;<span tabindex="0">T&lowast;2=1.3(3)&thinsp;&thinsp;&mu;s</span>, and four-pulse dynamical decoupling already extends the spin-coherence time to&nbsp;<span tabindex="0">T2=0.30(8)&thinsp;&thinsp;ms</span>. Combined with transform-limited photons and integration into photonic nanostructures, our results make the&nbsp;<span tabindex="0">SnV</span>&nbsp;a competitive spin-photon building block for quantum networks.</p>