Enhanced photocatalytic hydrogen evolution from water by niobate single molecular sheets and ensembles.

We report single molecular sheets of niobate prepared by a simple bottom-up approach using hydrothermal synthesis of niobium ethoxide with the aid of triethanolamine as a structural modifier: the high kinetic stability of these molecular entities against self-assembly allows them to mix well with ot...

Full description

Bibliographic Details
Main Authors: Nakagawa, K, Jia, T, Zheng, W, Fairclough, S, Katoh, M, Sugiyama, S, Tsang, S
Format: Journal article
Language:English
Published: Royal Society of Chemistry 2014
_version_ 1826300948134232064
author Nakagawa, K
Jia, T
Zheng, W
Fairclough, S
Katoh, M
Sugiyama, S
Tsang, S
author_facet Nakagawa, K
Jia, T
Zheng, W
Fairclough, S
Katoh, M
Sugiyama, S
Tsang, S
author_sort Nakagawa, K
collection OXFORD
description We report single molecular sheets of niobate prepared by a simple bottom-up approach using hydrothermal synthesis of niobium ethoxide with the aid of triethanolamine as a structural modifier: the high kinetic stability of these molecular entities against self-assembly allows them to mix well with other colloids and facilitates their extensive electronic interactions and thus photocatalytic hydrogen evolution activity from water is much enhanced over composite of single niobate sheets with graphene and MoS2 due to efficient electron transfer and charge separation.
first_indexed 2024-03-07T05:24:55Z
format Journal article
id oxford-uuid:e036c60f-ca80-4254-b868-bcfc79bbab1c
institution University of Oxford
language English
last_indexed 2024-03-07T05:24:55Z
publishDate 2014
publisher Royal Society of Chemistry
record_format dspace
spelling oxford-uuid:e036c60f-ca80-4254-b868-bcfc79bbab1c2022-03-27T09:45:25ZEnhanced photocatalytic hydrogen evolution from water by niobate single molecular sheets and ensembles.Journal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:e036c60f-ca80-4254-b868-bcfc79bbab1cEnglishSymplectic Elements at OxfordRoyal Society of Chemistry2014Nakagawa, KJia, TZheng, WFairclough, SKatoh, MSugiyama, STsang, SWe report single molecular sheets of niobate prepared by a simple bottom-up approach using hydrothermal synthesis of niobium ethoxide with the aid of triethanolamine as a structural modifier: the high kinetic stability of these molecular entities against self-assembly allows them to mix well with other colloids and facilitates their extensive electronic interactions and thus photocatalytic hydrogen evolution activity from water is much enhanced over composite of single niobate sheets with graphene and MoS2 due to efficient electron transfer and charge separation.
spellingShingle Nakagawa, K
Jia, T
Zheng, W
Fairclough, S
Katoh, M
Sugiyama, S
Tsang, S
Enhanced photocatalytic hydrogen evolution from water by niobate single molecular sheets and ensembles.
title Enhanced photocatalytic hydrogen evolution from water by niobate single molecular sheets and ensembles.
title_full Enhanced photocatalytic hydrogen evolution from water by niobate single molecular sheets and ensembles.
title_fullStr Enhanced photocatalytic hydrogen evolution from water by niobate single molecular sheets and ensembles.
title_full_unstemmed Enhanced photocatalytic hydrogen evolution from water by niobate single molecular sheets and ensembles.
title_short Enhanced photocatalytic hydrogen evolution from water by niobate single molecular sheets and ensembles.
title_sort enhanced photocatalytic hydrogen evolution from water by niobate single molecular sheets and ensembles
work_keys_str_mv AT nakagawak enhancedphotocatalytichydrogenevolutionfromwaterbyniobatesinglemolecularsheetsandensembles
AT jiat enhancedphotocatalytichydrogenevolutionfromwaterbyniobatesinglemolecularsheetsandensembles
AT zhengw enhancedphotocatalytichydrogenevolutionfromwaterbyniobatesinglemolecularsheetsandensembles
AT faircloughs enhancedphotocatalytichydrogenevolutionfromwaterbyniobatesinglemolecularsheetsandensembles
AT katohm enhancedphotocatalytichydrogenevolutionfromwaterbyniobatesinglemolecularsheetsandensembles
AT sugiyamas enhancedphotocatalytichydrogenevolutionfromwaterbyniobatesinglemolecularsheetsandensembles
AT tsangs enhancedphotocatalytichydrogenevolutionfromwaterbyniobatesinglemolecularsheetsandensembles