Angle-dependent magnetoresistance oscillations and Fermi surface reordering at high magnetic fields in α-(ET)2KHg(SCN)4

Angle dependent magnetoresistance oscillations (AMRO) have been studied in the charge transfer salt α-(ET)2KHg(SCN)4 for magnetic fields in the range 0 - 30 T. This salt exhibits the onset of antiferromagnetic order at temperatures TN approx.8-10 K and the presence below this temperature of a region...

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Main Authors: Caulfield, J, Blundell, S, Singleton, J, House, A, du Croo de Jongh, M, Hendriks, P, Perenboom, J, Hayes, W, Kurmoo, M, Day, P
Format: Journal article
Language:English
Published: Elsevier 1995
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author Caulfield, J
Blundell, S
Singleton, J
House, A
du Croo de Jongh, M
Hendriks, P
Perenboom, J
Hayes, W
Kurmoo, M
Day, P
author_facet Caulfield, J
Blundell, S
Singleton, J
House, A
du Croo de Jongh, M
Hendriks, P
Perenboom, J
Hayes, W
Kurmoo, M
Day, P
author_sort Caulfield, J
collection OXFORD
description Angle dependent magnetoresistance oscillations (AMRO) have been studied in the charge transfer salt α-(ET)2KHg(SCN)4 for magnetic fields in the range 0 - 30 T. This salt exhibits the onset of antiferromagnetic order at temperatures TN approx.8-10 K and the presence below this temperature of a region of sharp negative magnetoresistance at a field around 22 T known as the 'kink'. AMRO have been measured in this salt for a wide range of applied fields since the period, amplitude, and nature of the oscillations can be used to directly infer the character of the Fermi surface (FS) as a function of field. The data indicate that a profound change in the band structure occurs at this kink transition; the high field phase is characterised by quasi-2D oscillations from a closed cylindrical FS which is elongated in the c direction; the low field phase appears to be a spin density wave groundstate, with a FS consisting of a sheet (which is quasi-1D in character and tilted at an angle of approx.21° to the b*c plane) and small closed 2D pockets. It is suggested that the breakdown orbits between the pockets and the 1D sheets are able to account for the various Shubnikov-de Haas frequencies observed below the kink.
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spelling oxford-uuid:e1a016d5-6102-40ed-aa92-8b19cdbd56282022-03-27T09:55:50ZAngle-dependent magnetoresistance oscillations and Fermi surface reordering at high magnetic fields in α-(ET)2KHg(SCN)4 Journal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:e1a016d5-6102-40ed-aa92-8b19cdbd5628EnglishSymplectic Elements at OxfordElsevier1995Caulfield, JBlundell, SSingleton, JHouse, Adu Croo de Jongh, MHendriks, PPerenboom, JHayes, WKurmoo, MDay, PAngle dependent magnetoresistance oscillations (AMRO) have been studied in the charge transfer salt α-(ET)2KHg(SCN)4 for magnetic fields in the range 0 - 30 T. This salt exhibits the onset of antiferromagnetic order at temperatures TN approx.8-10 K and the presence below this temperature of a region of sharp negative magnetoresistance at a field around 22 T known as the 'kink'. AMRO have been measured in this salt for a wide range of applied fields since the period, amplitude, and nature of the oscillations can be used to directly infer the character of the Fermi surface (FS) as a function of field. The data indicate that a profound change in the band structure occurs at this kink transition; the high field phase is characterised by quasi-2D oscillations from a closed cylindrical FS which is elongated in the c direction; the low field phase appears to be a spin density wave groundstate, with a FS consisting of a sheet (which is quasi-1D in character and tilted at an angle of approx.21° to the b*c plane) and small closed 2D pockets. It is suggested that the breakdown orbits between the pockets and the 1D sheets are able to account for the various Shubnikov-de Haas frequencies observed below the kink.
spellingShingle Caulfield, J
Blundell, S
Singleton, J
House, A
du Croo de Jongh, M
Hendriks, P
Perenboom, J
Hayes, W
Kurmoo, M
Day, P
Angle-dependent magnetoresistance oscillations and Fermi surface reordering at high magnetic fields in α-(ET)2KHg(SCN)4
title Angle-dependent magnetoresistance oscillations and Fermi surface reordering at high magnetic fields in α-(ET)2KHg(SCN)4
title_full Angle-dependent magnetoresistance oscillations and Fermi surface reordering at high magnetic fields in α-(ET)2KHg(SCN)4
title_fullStr Angle-dependent magnetoresistance oscillations and Fermi surface reordering at high magnetic fields in α-(ET)2KHg(SCN)4
title_full_unstemmed Angle-dependent magnetoresistance oscillations and Fermi surface reordering at high magnetic fields in α-(ET)2KHg(SCN)4
title_short Angle-dependent magnetoresistance oscillations and Fermi surface reordering at high magnetic fields in α-(ET)2KHg(SCN)4
title_sort angle dependent magnetoresistance oscillations and fermi surface reordering at high magnetic fields in α et 2khg scn 4
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