Broadband impulsive vibrational spectroscopy of excited electronic states in the time domain

We demonstrate that transient absorption spectroscopy performed with an ultrashort pump pulse and a chirped, broad-band probe pulse is capable of recording full vibrational spectra of excited electronic states in the time domain. The resulting spectra do not suffer from the nontrivial baselines and...

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Bibliographic Details
Main Authors: Liebel, M, Kukura, P
Format: Journal article
Language:English
Published: American Chemical Society 2013