Localised polymer networks in chiral nematic liquid crystals for high speed photonic switching

Self-assembled periodic structures based upon chiralliquid crystalline materials have significant potential in the field of photonics ranging from fast-switching optoelectronic devices to low-threshold lasers. The flexoelectro-optic effect, which is observed in chiralnematic liquid crystals (LCs) wh...

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Main Authors: Tartan, C, Salter, P, Booth, M, Morris, S, Elston, S
Format: Journal article
Published: American Institute of Physics 2016
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author Tartan, C
Salter, P
Booth, M
Morris, S
Elston, S
author_facet Tartan, C
Salter, P
Booth, M
Morris, S
Elston, S
author_sort Tartan, C
collection OXFORD
description Self-assembled periodic structures based upon chiralliquid crystalline materials have significant potential in the field of photonics ranging from fast-switching optoelectronic devices to low-threshold lasers. The flexoelectro-optic effect, which is observed in chiralnematic liquid crystals (LCs) when an electric field is applied perpendicular to the helical axis, has significant potential as it exhibits analogue switching in 10–100 μs. However, the major technological barrier that prohibits the commercial realisation of this electro-opticeffect is the requirement of a uniform, in-plane alignment of the helix axis between glass substrates. Here, it is shown that periodic polymer structures engineered in the nematic phase of a chiral nematic LC device using direct laser writing can result in the spontaneous formation of the necessary uniform lying helix (ULH) state. Specifically, two-photon polymerization is used in conjunction with a spatial light modulator so as to correct for aberrations introduced by the bounding glass substrates enabling the polymer structures to be fabricated directly into the device. The ULH state appears to be stable in the absence of an externally applied electric field, and the optimum contrast between the bright and dark states is obtained using polymer structures that have periodicities of the order of the device thickness.
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spelling oxford-uuid:f7147672-be9b-4e84-bb05-43725485e4d52022-03-27T12:40:01ZLocalised polymer networks in chiral nematic liquid crystals for high speed photonic switchingJournal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:f7147672-be9b-4e84-bb05-43725485e4d5Symplectic Elements at OxfordAmerican Institute of Physics2016Tartan, CSalter, PBooth, MMorris, SElston, SSelf-assembled periodic structures based upon chiralliquid crystalline materials have significant potential in the field of photonics ranging from fast-switching optoelectronic devices to low-threshold lasers. The flexoelectro-optic effect, which is observed in chiralnematic liquid crystals (LCs) when an electric field is applied perpendicular to the helical axis, has significant potential as it exhibits analogue switching in 10–100 μs. However, the major technological barrier that prohibits the commercial realisation of this electro-opticeffect is the requirement of a uniform, in-plane alignment of the helix axis between glass substrates. Here, it is shown that periodic polymer structures engineered in the nematic phase of a chiral nematic LC device using direct laser writing can result in the spontaneous formation of the necessary uniform lying helix (ULH) state. Specifically, two-photon polymerization is used in conjunction with a spatial light modulator so as to correct for aberrations introduced by the bounding glass substrates enabling the polymer structures to be fabricated directly into the device. The ULH state appears to be stable in the absence of an externally applied electric field, and the optimum contrast between the bright and dark states is obtained using polymer structures that have periodicities of the order of the device thickness.
spellingShingle Tartan, C
Salter, P
Booth, M
Morris, S
Elston, S
Localised polymer networks in chiral nematic liquid crystals for high speed photonic switching
title Localised polymer networks in chiral nematic liquid crystals for high speed photonic switching
title_full Localised polymer networks in chiral nematic liquid crystals for high speed photonic switching
title_fullStr Localised polymer networks in chiral nematic liquid crystals for high speed photonic switching
title_full_unstemmed Localised polymer networks in chiral nematic liquid crystals for high speed photonic switching
title_short Localised polymer networks in chiral nematic liquid crystals for high speed photonic switching
title_sort localised polymer networks in chiral nematic liquid crystals for high speed photonic switching
work_keys_str_mv AT tartanc localisedpolymernetworksinchiralnematicliquidcrystalsforhighspeedphotonicswitching
AT salterp localisedpolymernetworksinchiralnematicliquidcrystalsforhighspeedphotonicswitching
AT boothm localisedpolymernetworksinchiralnematicliquidcrystalsforhighspeedphotonicswitching
AT morriss localisedpolymernetworksinchiralnematicliquidcrystalsforhighspeedphotonicswitching
AT elstons localisedpolymernetworksinchiralnematicliquidcrystalsforhighspeedphotonicswitching