Biocomposite of cassava starch-cymbopogan citratus fibre: Mechanical, thermal and biodegradation properties

Increasing environmental awareness and concern have shifted the focus of research and development towards biodegradable materials development. In the current study, Cymbopogan citratus fibre (CCF) were incorporated into thermoplastic cassava starch (TPCS) with various content of CCF (10, 20, 30, 40,...

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Main Authors: Zatil Hafila Kamaruddin, Ridhwan Jumaidin, Rushdan Ahmad Ilyas, Mohd Zulkefli Selamat, Roziela Hanim Alamjuri, Fahmi Asyadi Md Yusof
Format: Article
Language:English
English
Published: MDPI 2022
Subjects:
Online Access:https://eprints.ums.edu.my/id/eprint/33411/2/Biocomposite%20of%20cassava%20starch-cymbopogan%20citratus%20fibre%2C%20Mechanical%2C%20thermal%20and%20biodegradation%20properties.ABSTRACT.pdf
https://eprints.ums.edu.my/id/eprint/33411/1/Biocomposite%20of%20Cassava%20Starch-Cymbopogan%20Citratus%20Fibre%2C%20Mechanical%2C%20Thermal%20and%20Biodegradation%20Properties.pdf
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author Zatil Hafila Kamaruddin
Ridhwan Jumaidin
Rushdan Ahmad Ilyas
Mohd Zulkefli Selamat
Roziela Hanim Alamjuri
Fahmi Asyadi Md Yusof
author_facet Zatil Hafila Kamaruddin
Ridhwan Jumaidin
Rushdan Ahmad Ilyas
Mohd Zulkefli Selamat
Roziela Hanim Alamjuri
Fahmi Asyadi Md Yusof
author_sort Zatil Hafila Kamaruddin
collection UMS
description Increasing environmental awareness and concern have shifted the focus of research and development towards biodegradable materials development. In the current study, Cymbopogan citratus fibre (CCF) were incorporated into thermoplastic cassava starch (TPCS) with various content of CCF (10, 20, 30, 40, 50, 60 wt.%) via compression moulding. The determination of fundamental characteristics of TPCS/CCF biopolymer composites was conducted to assess their potential as biodegradable reinforcements. Characterization of the samples was conducted via Fourier-transform infrared spectroscopy (FT-IR), thermogravimetric analysis (TGA), and scanning electron microscopy (SEM), as well as mechanical, moisture absorption, and soil burial testings. The findings showed that the improved tensile and flexural features of the TPCS composites with CCF incorporation, with 50 wt.% CCF content yielded the maximum modulus and strength. The thermal properties of the biocomposite demonstrated that CCF addition improved the material’s thermal stability, as shown by a higher-onset decomposition temperature and ash content. Meanwhile, the CCF incorporation into TPCS slowed down the biodegradation of the composites. In term of morphological, homoge-neous fibres and matrix dispersion with excellent adhesion was observed in morphological analyses using scanning electron microscopy (SEM), which is crucial for the enhancement of the mechanical performance of biocomposites.
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spelling ums.eprints-334112022-07-21T01:03:36Z https://eprints.ums.edu.my/id/eprint/33411/ Biocomposite of cassava starch-cymbopogan citratus fibre: Mechanical, thermal and biodegradation properties Zatil Hafila Kamaruddin Ridhwan Jumaidin Rushdan Ahmad Ilyas Mohd Zulkefli Selamat Roziela Hanim Alamjuri Fahmi Asyadi Md Yusof TP200-248 Chemicals: Manufacture, use, etc. Increasing environmental awareness and concern have shifted the focus of research and development towards biodegradable materials development. In the current study, Cymbopogan citratus fibre (CCF) were incorporated into thermoplastic cassava starch (TPCS) with various content of CCF (10, 20, 30, 40, 50, 60 wt.%) via compression moulding. The determination of fundamental characteristics of TPCS/CCF biopolymer composites was conducted to assess their potential as biodegradable reinforcements. Characterization of the samples was conducted via Fourier-transform infrared spectroscopy (FT-IR), thermogravimetric analysis (TGA), and scanning electron microscopy (SEM), as well as mechanical, moisture absorption, and soil burial testings. The findings showed that the improved tensile and flexural features of the TPCS composites with CCF incorporation, with 50 wt.% CCF content yielded the maximum modulus and strength. The thermal properties of the biocomposite demonstrated that CCF addition improved the material’s thermal stability, as shown by a higher-onset decomposition temperature and ash content. Meanwhile, the CCF incorporation into TPCS slowed down the biodegradation of the composites. In term of morphological, homoge-neous fibres and matrix dispersion with excellent adhesion was observed in morphological analyses using scanning electron microscopy (SEM), which is crucial for the enhancement of the mechanical performance of biocomposites. MDPI 2022-01-27 Article NonPeerReviewed text en https://eprints.ums.edu.my/id/eprint/33411/2/Biocomposite%20of%20cassava%20starch-cymbopogan%20citratus%20fibre%2C%20Mechanical%2C%20thermal%20and%20biodegradation%20properties.ABSTRACT.pdf text en https://eprints.ums.edu.my/id/eprint/33411/1/Biocomposite%20of%20Cassava%20Starch-Cymbopogan%20Citratus%20Fibre%2C%20Mechanical%2C%20Thermal%20and%20Biodegradation%20Properties.pdf Zatil Hafila Kamaruddin and Ridhwan Jumaidin and Rushdan Ahmad Ilyas and Mohd Zulkefli Selamat and Roziela Hanim Alamjuri and Fahmi Asyadi Md Yusof (2022) Biocomposite of cassava starch-cymbopogan citratus fibre: Mechanical, thermal and biodegradation properties. Polymers, 14. pp. 1-19. ISSN 2073-4360 https://www.mdpi.com/2073-4360/14/3/514/pdf https://doi.10.3390/polym14030514 https://doi.10.3390/polym14030514
spellingShingle TP200-248 Chemicals: Manufacture, use, etc.
Zatil Hafila Kamaruddin
Ridhwan Jumaidin
Rushdan Ahmad Ilyas
Mohd Zulkefli Selamat
Roziela Hanim Alamjuri
Fahmi Asyadi Md Yusof
Biocomposite of cassava starch-cymbopogan citratus fibre: Mechanical, thermal and biodegradation properties
title Biocomposite of cassava starch-cymbopogan citratus fibre: Mechanical, thermal and biodegradation properties
title_full Biocomposite of cassava starch-cymbopogan citratus fibre: Mechanical, thermal and biodegradation properties
title_fullStr Biocomposite of cassava starch-cymbopogan citratus fibre: Mechanical, thermal and biodegradation properties
title_full_unstemmed Biocomposite of cassava starch-cymbopogan citratus fibre: Mechanical, thermal and biodegradation properties
title_short Biocomposite of cassava starch-cymbopogan citratus fibre: Mechanical, thermal and biodegradation properties
title_sort biocomposite of cassava starch cymbopogan citratus fibre mechanical thermal and biodegradation properties
topic TP200-248 Chemicals: Manufacture, use, etc.
url https://eprints.ums.edu.my/id/eprint/33411/2/Biocomposite%20of%20cassava%20starch-cymbopogan%20citratus%20fibre%2C%20Mechanical%2C%20thermal%20and%20biodegradation%20properties.ABSTRACT.pdf
https://eprints.ums.edu.my/id/eprint/33411/1/Biocomposite%20of%20Cassava%20Starch-Cymbopogan%20Citratus%20Fibre%2C%20Mechanical%2C%20Thermal%20and%20Biodegradation%20Properties.pdf
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