Removal of remazol red dyes using zeolites-loaded nanofibre coated on fabric substrates

Nanofibre-based membranes have shown great potential for removing textile wastewater due to their high porosity and surface area. However, nanofibre membranes exhibit lower dye removal efficiency. Hence, this study aims to improve the dye removal performance of nanofibre membranes by incorporating z...

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Main Authors: Siddratul Sarah Binti Mohd Hami, Nor Dalila Nor Affandi, Liliana Indrie, Ahmad Mukifza Harun
Format: Article
Language:English
English
Published: Multidisciplinary Digital Publishing Institute (MDPI) 2024
Subjects:
Online Access:https://eprints.ums.edu.my/id/eprint/42089/1/ABSTRACT.pdf
https://eprints.ums.edu.my/id/eprint/42089/2/FULL%20TEXT.pdf
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author Siddratul Sarah Binti Mohd Hami
Nor Dalila Nor Affandi
Liliana Indrie
Ahmad Mukifza Harun
author_facet Siddratul Sarah Binti Mohd Hami
Nor Dalila Nor Affandi
Liliana Indrie
Ahmad Mukifza Harun
author_sort Siddratul Sarah Binti Mohd Hami
collection UMS
description Nanofibre-based membranes have shown great potential for removing textile wastewater due to their high porosity and surface area. However, nanofibre membranes exhibit lower dye removal efficiency. Hence, this study aims to improve the dye removal performance of nanofibre membranes by incorporating zeolites. The research involved fabricating composite membranes by electrospinning polyvinyl alcohol (PVA) nanofibres incorporated with zeolites. Mechanical strength was enhanced by placing the PVA/zeolite nanofibre membrane between fusible nonwoven interfacing and woven polyester fabric, followed by heat treatment. Morphological analysis revealed the uniform dispersion of zeolite particles within the PVA nanofibres. EDX analysis confirmed the successful incorporation of zeolites into the fibres. Among all membrane samples, the PZ-0.75 membrane exhibited the highest pure water flux (PWF) with approximately 1358.57 L·m−2 ·min−1 for distilled water and 499.85 L·m−2 ·min−1 for batik wastewater. Turbidity of batik wastewater increased proportionally with zeolite concentration, with removal rates of 84.79%, 78.8%, 76.96%, and 74.19% for PZ-0.75, PZ-0.5, PZ-0.25, and PVA membranes, respectively. Furthermore, the UV/Vis spectrophotometer demonstrated that dye removal efficiency increased from 2.22% to 8.89% as the zeolite concentration increased from 0% to 0.75%. In addition, the PZ-0.75 membrane effectively removed RR dye at a concentration of 1 mg/L, with an optimal contact time of approximately 60 min. The adsorption mechanism of the PZ-0.75 membrane aligns with the Freundlich model, with an R2 value of 0.983. Overall, this study demonstrates the efficiency of zeolite in the fabric substrates to improve the filtration and adsorption properties for wastewater treatment, particularly in textile industries.
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spelling ums.eprints-420892024-12-04T07:20:06Z https://eprints.ums.edu.my/id/eprint/42089/ Removal of remazol red dyes using zeolites-loaded nanofibre coated on fabric substrates Siddratul Sarah Binti Mohd Hami Nor Dalila Nor Affandi Liliana Indrie Ahmad Mukifza Harun TA401-492 Materials of engineering and construction. Mechanics of materials TD511-780 Sewage collection and disposal systems. Sewerage Nanofibre-based membranes have shown great potential for removing textile wastewater due to their high porosity and surface area. However, nanofibre membranes exhibit lower dye removal efficiency. Hence, this study aims to improve the dye removal performance of nanofibre membranes by incorporating zeolites. The research involved fabricating composite membranes by electrospinning polyvinyl alcohol (PVA) nanofibres incorporated with zeolites. Mechanical strength was enhanced by placing the PVA/zeolite nanofibre membrane between fusible nonwoven interfacing and woven polyester fabric, followed by heat treatment. Morphological analysis revealed the uniform dispersion of zeolite particles within the PVA nanofibres. EDX analysis confirmed the successful incorporation of zeolites into the fibres. Among all membrane samples, the PZ-0.75 membrane exhibited the highest pure water flux (PWF) with approximately 1358.57 L·m−2 ·min−1 for distilled water and 499.85 L·m−2 ·min−1 for batik wastewater. Turbidity of batik wastewater increased proportionally with zeolite concentration, with removal rates of 84.79%, 78.8%, 76.96%, and 74.19% for PZ-0.75, PZ-0.5, PZ-0.25, and PVA membranes, respectively. Furthermore, the UV/Vis spectrophotometer demonstrated that dye removal efficiency increased from 2.22% to 8.89% as the zeolite concentration increased from 0% to 0.75%. In addition, the PZ-0.75 membrane effectively removed RR dye at a concentration of 1 mg/L, with an optimal contact time of approximately 60 min. The adsorption mechanism of the PZ-0.75 membrane aligns with the Freundlich model, with an R2 value of 0.983. Overall, this study demonstrates the efficiency of zeolite in the fabric substrates to improve the filtration and adsorption properties for wastewater treatment, particularly in textile industries. Multidisciplinary Digital Publishing Institute (MDPI) 2024 Article NonPeerReviewed text en https://eprints.ums.edu.my/id/eprint/42089/1/ABSTRACT.pdf text en https://eprints.ums.edu.my/id/eprint/42089/2/FULL%20TEXT.pdf Siddratul Sarah Binti Mohd Hami and Nor Dalila Nor Affandi and Liliana Indrie and Ahmad Mukifza Harun (2024) Removal of remazol red dyes using zeolites-loaded nanofibre coated on fabric substrates. Coatings, 14. pp. 1-16. https://doi.org/10.3390/coatings14091155
spellingShingle TA401-492 Materials of engineering and construction. Mechanics of materials
TD511-780 Sewage collection and disposal systems. Sewerage
Siddratul Sarah Binti Mohd Hami
Nor Dalila Nor Affandi
Liliana Indrie
Ahmad Mukifza Harun
Removal of remazol red dyes using zeolites-loaded nanofibre coated on fabric substrates
title Removal of remazol red dyes using zeolites-loaded nanofibre coated on fabric substrates
title_full Removal of remazol red dyes using zeolites-loaded nanofibre coated on fabric substrates
title_fullStr Removal of remazol red dyes using zeolites-loaded nanofibre coated on fabric substrates
title_full_unstemmed Removal of remazol red dyes using zeolites-loaded nanofibre coated on fabric substrates
title_short Removal of remazol red dyes using zeolites-loaded nanofibre coated on fabric substrates
title_sort removal of remazol red dyes using zeolites loaded nanofibre coated on fabric substrates
topic TA401-492 Materials of engineering and construction. Mechanics of materials
TD511-780 Sewage collection and disposal systems. Sewerage
url https://eprints.ums.edu.my/id/eprint/42089/1/ABSTRACT.pdf
https://eprints.ums.edu.my/id/eprint/42089/2/FULL%20TEXT.pdf
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AT nordalilanoraffandi removalofremazolreddyesusingzeolitesloadednanofibrecoatedonfabricsubstrates
AT lilianaindrie removalofremazolreddyesusingzeolitesloadednanofibrecoatedonfabricsubstrates
AT ahmadmukifzaharun removalofremazolreddyesusingzeolitesloadednanofibrecoatedonfabricsubstrates