A new reactor concept for combining oxidative coupling and steam re-forming of methane: modeling and analysis

A new and very promising application of auto-thermal reactors is the coupling of endothermic and exothermic reactions where the product of the endothermic reaction is the desired one. Therefore, in this work, a reactor in which oxidative coupling of methane (OCM) and steam re-forming of methane (SRM...

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Main Authors: Farsi, Ali, Shadravan, Vahid, Mansouri, Seyed Sohil, Zahedi, Gholamreza, Abdul Manan, Zainuddin
Format: Article
Published: John Wiley and Sons Ltd 2013
Subjects:
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author Farsi, Ali
Shadravan, Vahid
Mansouri, Seyed Sohil
Zahedi, Gholamreza
Abdul Manan, Zainuddin
author_facet Farsi, Ali
Shadravan, Vahid
Mansouri, Seyed Sohil
Zahedi, Gholamreza
Abdul Manan, Zainuddin
author_sort Farsi, Ali
collection ePrints
description A new and very promising application of auto-thermal reactors is the coupling of endothermic and exothermic reactions where the product of the endothermic reaction is the desired one. Therefore, in this work, a reactor in which oxidative coupling of methane (OCM) and steam re-forming of methane (SRM) reactions take place simultaneously was modeled. The results were obtained in a wide range of different conditions such as inlet feed, inlet temperature, portions of OCM and SRM catalysts, and inlet velocity. In selection of the catalysts, more attention was drawn to prevent re-forming of OCM products. The main parameters of each reaction under different conditions such as conversion of the feed components, products selectivity and yield, temperature in the length of reactor, and component's concentration in the reactor were considered in course of this study. The results revealed that simultaneous OCM and SRM reactions in one reactor will tend to be auto-thermal, and the waste of energy will be reduced. The results also show that complete conversion of water and majority of methane and oxygen will decrease the amount of unwanted products at the reactor's discharge-a constraint that exists in single reactors of each reaction specially OCM.
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spelling utm.eprints-285892019-01-28T03:35:24Z http://eprints.utm.my/28589/ A new reactor concept for combining oxidative coupling and steam re-forming of methane: modeling and analysis Farsi, Ali Shadravan, Vahid Mansouri, Seyed Sohil Zahedi, Gholamreza Abdul Manan, Zainuddin QD Chemistry TP Chemical technology A new and very promising application of auto-thermal reactors is the coupling of endothermic and exothermic reactions where the product of the endothermic reaction is the desired one. Therefore, in this work, a reactor in which oxidative coupling of methane (OCM) and steam re-forming of methane (SRM) reactions take place simultaneously was modeled. The results were obtained in a wide range of different conditions such as inlet feed, inlet temperature, portions of OCM and SRM catalysts, and inlet velocity. In selection of the catalysts, more attention was drawn to prevent re-forming of OCM products. The main parameters of each reaction under different conditions such as conversion of the feed components, products selectivity and yield, temperature in the length of reactor, and component's concentration in the reactor were considered in course of this study. The results revealed that simultaneous OCM and SRM reactions in one reactor will tend to be auto-thermal, and the waste of energy will be reduced. The results also show that complete conversion of water and majority of methane and oxygen will decrease the amount of unwanted products at the reactor's discharge-a constraint that exists in single reactors of each reaction specially OCM. John Wiley and Sons Ltd 2013-02 Article PeerReviewed Farsi, Ali and Shadravan, Vahid and Mansouri, Seyed Sohil and Zahedi, Gholamreza and Abdul Manan, Zainuddin (2013) A new reactor concept for combining oxidative coupling and steam re-forming of methane: modeling and analysis. International Journal of Energy Research, 37 (2). pp. 129-152. ISSN 0363-907X http://dx.doi.org/10.1002/er.1881 DOI:10.1002/er.1881
spellingShingle QD Chemistry
TP Chemical technology
Farsi, Ali
Shadravan, Vahid
Mansouri, Seyed Sohil
Zahedi, Gholamreza
Abdul Manan, Zainuddin
A new reactor concept for combining oxidative coupling and steam re-forming of methane: modeling and analysis
title A new reactor concept for combining oxidative coupling and steam re-forming of methane: modeling and analysis
title_full A new reactor concept for combining oxidative coupling and steam re-forming of methane: modeling and analysis
title_fullStr A new reactor concept for combining oxidative coupling and steam re-forming of methane: modeling and analysis
title_full_unstemmed A new reactor concept for combining oxidative coupling and steam re-forming of methane: modeling and analysis
title_short A new reactor concept for combining oxidative coupling and steam re-forming of methane: modeling and analysis
title_sort new reactor concept for combining oxidative coupling and steam re forming of methane modeling and analysis
topic QD Chemistry
TP Chemical technology
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