Ni–Pt/Al nano-sized catalyst supported on TNPs for hydrogen and valuable fuel production from the steam reforming of plastic waste dissolved in phenol
In this research, titanium nanoparticles (TNPs) for Ni–Pt/Al nano-sized catalysts were prepared via the hydrothermal technique, and their catalytic performance for the polyethylene terephthalate (PET) as plastic waste and phenol steam reforming reaction was examined. Complementary characterization m...
| Main Authors: | , , , , , , , , |
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| Format: | Article |
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Elsevier Ltd.
2020
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| _version_ | 1796865589692596224 |
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| author | Nabgan, Walid Nabgan, Bahador Tuan Abdullah, Tuan Amran Alqaraghuli, Hasan Ngadi, Norzita Abdul Jalil, Aishah Othman, Bashar Mohammed Ibrahim, Ammar Mahmoud Tan, Ji Siang |
| author_facet | Nabgan, Walid Nabgan, Bahador Tuan Abdullah, Tuan Amran Alqaraghuli, Hasan Ngadi, Norzita Abdul Jalil, Aishah Othman, Bashar Mohammed Ibrahim, Ammar Mahmoud Tan, Ji Siang |
| author_sort | Nabgan, Walid |
| collection | ePrints |
| description | In this research, titanium nanoparticles (TNPs) for Ni–Pt/Al nano-sized catalysts were prepared via the hydrothermal technique, and their catalytic performance for the polyethylene terephthalate (PET) as plastic waste and phenol steam reforming reaction was examined. Complementary characterization methods, such as BET, ICP, TEM, XRD, FTIR, NH3-TPD, H2-TPR, CO2-TPD, TGA, and CHNS, were conducted to relate surface functionality and structure to the activity of catalysts. The catalytic activity and stability with ten days on stream at 700 °C were investigated. It was found that the catalyst properties such as surface area and the number of acid sites play a crucial role in catalyst activity. The feed conversion and hydrogen yield for the optimum catalyst that is Ni–Pt/Ti–Al were found to be 92% and 75%, respectively. This research has also emphasized the opportunities of this method to resolve the threat of PET plastic waste to the environment concerning the creation of valuable fuels such as benzene, toluene, styrene, methylindene, etc. |
| first_indexed | 2024-03-05T20:59:18Z |
| format | Article |
| id | utm.eprints-93275 |
| institution | Universiti Teknologi Malaysia - ePrints |
| last_indexed | 2024-03-05T20:59:18Z |
| publishDate | 2020 |
| publisher | Elsevier Ltd. |
| record_format | dspace |
| spelling | utm.eprints-932752021-11-19T03:29:57Z http://eprints.utm.my/93275/ Ni–Pt/Al nano-sized catalyst supported on TNPs for hydrogen and valuable fuel production from the steam reforming of plastic waste dissolved in phenol Nabgan, Walid Nabgan, Bahador Tuan Abdullah, Tuan Amran Alqaraghuli, Hasan Ngadi, Norzita Abdul Jalil, Aishah Othman, Bashar Mohammed Ibrahim, Ammar Mahmoud Tan, Ji Siang TP Chemical technology In this research, titanium nanoparticles (TNPs) for Ni–Pt/Al nano-sized catalysts were prepared via the hydrothermal technique, and their catalytic performance for the polyethylene terephthalate (PET) as plastic waste and phenol steam reforming reaction was examined. Complementary characterization methods, such as BET, ICP, TEM, XRD, FTIR, NH3-TPD, H2-TPR, CO2-TPD, TGA, and CHNS, were conducted to relate surface functionality and structure to the activity of catalysts. The catalytic activity and stability with ten days on stream at 700 °C were investigated. It was found that the catalyst properties such as surface area and the number of acid sites play a crucial role in catalyst activity. The feed conversion and hydrogen yield for the optimum catalyst that is Ni–Pt/Ti–Al were found to be 92% and 75%, respectively. This research has also emphasized the opportunities of this method to resolve the threat of PET plastic waste to the environment concerning the creation of valuable fuels such as benzene, toluene, styrene, methylindene, etc. Elsevier Ltd. 2020-09-03 Article PeerReviewed Nabgan, Walid and Nabgan, Bahador and Tuan Abdullah, Tuan Amran and Alqaraghuli, Hasan and Ngadi, Norzita and Abdul Jalil, Aishah and Othman, Bashar Mohammed and Ibrahim, Ammar Mahmoud and Tan, Ji Siang (2020) Ni–Pt/Al nano-sized catalyst supported on TNPs for hydrogen and valuable fuel production from the steam reforming of plastic waste dissolved in phenol. International Journal of Hydrogen Energy, 45 (43). pp. 22817-22832. ISSN 0360-3199 http://dx.doi.org/10.1016/j.ijhydene.2020.06.128 DOI:10.1016/j.ijhydene.2020.06.128 |
| spellingShingle | TP Chemical technology Nabgan, Walid Nabgan, Bahador Tuan Abdullah, Tuan Amran Alqaraghuli, Hasan Ngadi, Norzita Abdul Jalil, Aishah Othman, Bashar Mohammed Ibrahim, Ammar Mahmoud Tan, Ji Siang Ni–Pt/Al nano-sized catalyst supported on TNPs for hydrogen and valuable fuel production from the steam reforming of plastic waste dissolved in phenol |
| title | Ni–Pt/Al nano-sized catalyst supported on TNPs for hydrogen and valuable fuel production from the steam reforming of plastic waste dissolved in phenol |
| title_full | Ni–Pt/Al nano-sized catalyst supported on TNPs for hydrogen and valuable fuel production from the steam reforming of plastic waste dissolved in phenol |
| title_fullStr | Ni–Pt/Al nano-sized catalyst supported on TNPs for hydrogen and valuable fuel production from the steam reforming of plastic waste dissolved in phenol |
| title_full_unstemmed | Ni–Pt/Al nano-sized catalyst supported on TNPs for hydrogen and valuable fuel production from the steam reforming of plastic waste dissolved in phenol |
| title_short | Ni–Pt/Al nano-sized catalyst supported on TNPs for hydrogen and valuable fuel production from the steam reforming of plastic waste dissolved in phenol |
| title_sort | ni pt al nano sized catalyst supported on tnps for hydrogen and valuable fuel production from the steam reforming of plastic waste dissolved in phenol |
| topic | TP Chemical technology |
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