Effect of gas flow channel structure on the performance of an anode-supported honeycomb solid oxide fuel cell

An anode-supported honeycomb SOFC gives high volumetric power density and improves thermo-mechanical durability at high temperatures. We have so far fabricated and tested a honeycomb cell with a cathode layer of LSM and an electrolyte layer of 8YSZ on a porous anode honeycomb substrate of Ni/8YSZ. T...

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Main Authors: Hironori NAKAJIMA, Shunzaburo MURAKAMI, Tatsumi KITAHARA
Format: Article
Language:Japanese
Published: The Japan Society of Mechanical Engineers 2018-02-01
Series:Nihon Kikai Gakkai ronbunshu
Subjects:
Online Access:https://www.jstage.jst.go.jp/article/transjsme/84/859/84_17-00419/_pdf/-char/en
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author Hironori NAKAJIMA
Shunzaburo MURAKAMI
Tatsumi KITAHARA
author_facet Hironori NAKAJIMA
Shunzaburo MURAKAMI
Tatsumi KITAHARA
author_sort Hironori NAKAJIMA
collection DOAJ
description An anode-supported honeycomb SOFC gives high volumetric power density and improves thermo-mechanical durability at high temperatures. We have so far fabricated and tested a honeycomb cell with a cathode layer of LSM and an electrolyte layer of 8YSZ on a porous anode honeycomb substrate of Ni/8YSZ. The anode-supported honeycomb cell exhibited promising volumetric power densities. In the present study, current-voltage and current-volumetric power density characteristics of the cells having different flow channel arrangements of the anode and cathode are measured under various inlet hydrogen fuel flow rates to show the effect of three-dimensional transport and distribution of the fuel in the porous anode substrate on the cell performance. We measure ohmic resistances of the honeycomb cells by current interruption method, and indicate the impact of nickel catalyst re-oxidation in the anode substrate by the fuel depletion with the flow channel arrangements resulting in high ohmic resistances and deactivation of the nickel catalyst. In low inlet fuel flow rate, smaller number of the anode flow channel is thereby advantageous, while larger number of the anode flow channel is advantageous in high inlet fuel flow rate. We also discuss suitable flow channel arrangements depending on inlet fuel flow rate to choose an appropriate operation mode.
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spelling doaj.art-0e5b850a909e42fdabec1a129634c9f02022-12-22T04:35:11ZjpnThe Japan Society of Mechanical EngineersNihon Kikai Gakkai ronbunshu2187-97612018-02-018485917-0041917-0041910.1299/transjsme.17-00419transjsmeEffect of gas flow channel structure on the performance of an anode-supported honeycomb solid oxide fuel cellHironori NAKAJIMA0Shunzaburo MURAKAMI1Tatsumi KITAHARA2Department of Mechanical Engineering, Faculty of Engineering, Kyushu UniversityDepartment of Hydrogen Energy Systems, Graduate School of Engineering, Kyushu UniversityDepartment of Mechanical Engineering, Faculty of Engineering, Kyushu UniversityAn anode-supported honeycomb SOFC gives high volumetric power density and improves thermo-mechanical durability at high temperatures. We have so far fabricated and tested a honeycomb cell with a cathode layer of LSM and an electrolyte layer of 8YSZ on a porous anode honeycomb substrate of Ni/8YSZ. The anode-supported honeycomb cell exhibited promising volumetric power densities. In the present study, current-voltage and current-volumetric power density characteristics of the cells having different flow channel arrangements of the anode and cathode are measured under various inlet hydrogen fuel flow rates to show the effect of three-dimensional transport and distribution of the fuel in the porous anode substrate on the cell performance. We measure ohmic resistances of the honeycomb cells by current interruption method, and indicate the impact of nickel catalyst re-oxidation in the anode substrate by the fuel depletion with the flow channel arrangements resulting in high ohmic resistances and deactivation of the nickel catalyst. In low inlet fuel flow rate, smaller number of the anode flow channel is thereby advantageous, while larger number of the anode flow channel is advantageous in high inlet fuel flow rate. We also discuss suitable flow channel arrangements depending on inlet fuel flow rate to choose an appropriate operation mode.https://www.jstage.jst.go.jp/article/transjsme/84/859/84_17-00419/_pdf/-char/ensofchoneycombanode-supportporous substratefuel transportni re-oxidation
spellingShingle Hironori NAKAJIMA
Shunzaburo MURAKAMI
Tatsumi KITAHARA
Effect of gas flow channel structure on the performance of an anode-supported honeycomb solid oxide fuel cell
Nihon Kikai Gakkai ronbunshu
sofc
honeycomb
anode-support
porous substrate
fuel transport
ni re-oxidation
title Effect of gas flow channel structure on the performance of an anode-supported honeycomb solid oxide fuel cell
title_full Effect of gas flow channel structure on the performance of an anode-supported honeycomb solid oxide fuel cell
title_fullStr Effect of gas flow channel structure on the performance of an anode-supported honeycomb solid oxide fuel cell
title_full_unstemmed Effect of gas flow channel structure on the performance of an anode-supported honeycomb solid oxide fuel cell
title_short Effect of gas flow channel structure on the performance of an anode-supported honeycomb solid oxide fuel cell
title_sort effect of gas flow channel structure on the performance of an anode supported honeycomb solid oxide fuel cell
topic sofc
honeycomb
anode-support
porous substrate
fuel transport
ni re-oxidation
url https://www.jstage.jst.go.jp/article/transjsme/84/859/84_17-00419/_pdf/-char/en
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AT shunzaburomurakami effectofgasflowchannelstructureontheperformanceofananodesupportedhoneycombsolidoxidefuelcell
AT tatsumikitahara effectofgasflowchannelstructureontheperformanceofananodesupportedhoneycombsolidoxidefuelcell