Collision-Induced C_{60} Rovibrational Relaxation Probed by State-Resolved Nonlinear Spectroscopy

Quantum state-resolved spectroscopy was recently achieved for C_{60} molecules when cooled by buffer gas collisions and probed with a midinfrared frequency comb. This rovibrational quantum state resolution for the largest molecule on record is facilitated by the remarkable symmetry and rigidity of C...

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Bibliographic Details
Main Authors: Lee R. Liu, P. Bryan Changala, Marissa L. Weichman, Qizhong Liang, Jutta Toscano, Jacek Kłos, Svetlana Kotochigova, David J. Nesbitt, Jun Ye
Format: Article
Language:English
Published: American Physical Society 2022-09-01
Series:PRX Quantum
Online Access:http://doi.org/10.1103/PRXQuantum.3.030332