Absolute frequency metrology of buffer-gas-cooled molecular spectra at 1 kHz accuracy level

High-resolution molecular spectroscopy with cryogenic setups is hampered by the lack of a skilled interrogation tool. Here, the authors demonstrate absolute metrology of cold rovibrational spectra at 1 kHz accuracy level, by coupling a Lamb-dip saturated-absorption cavity ring-down spectrometer to a...

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Bibliographic Details
Main Authors: Roberto Aiello, Valentina Di Sarno, Maria Giulia Delli Santi, Maurizio De Rosa, Iolanda Ricciardi, Paolo De Natale, Luigi Santamaria, Giovanni Giusfredi, Pasquale Maddaloni
Format: Article
Language:English
Published: Nature Portfolio 2022-11-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-022-34758-9