Revealing the role of liquid preordering in crystallisation of supercooled liquids

In classical nucleation theory, structural order in the liquid phase is not considered. But simulations of supercooled liquids now show that crystal-like liquid preordering play an essential role in nucleation and growth processes - calling for extensions of the classical theory.

Bibliographic Details
Main Authors: Yuan-Chao Hu, Hajime Tanaka
Format: Article
Language:English
Published: Nature Portfolio 2022-08-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-022-32241-z