Temperature dependence of the band gap of ^{28}Si:P at very low temperatures measured via time-resolved optical spectroscopy

We measure the temperature dependence of the indirect band gap of isotopically purified ^{28}Si:P in the regime from 0.1 K to 3 K by high-resolution absorption spectroscopy of the donor bound exciton transition. The measurements increase the up-to-date precision of the temperature-dependent band gap...

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Main Authors: E. Sauter, N. V. Abrosimov, J. Hübner, M. Oestreich
Format: Article
Language:English
Published: American Physical Society 2023-03-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.5.013182
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author E. Sauter
N. V. Abrosimov
J. Hübner
M. Oestreich
author_facet E. Sauter
N. V. Abrosimov
J. Hübner
M. Oestreich
author_sort E. Sauter
collection DOAJ
description We measure the temperature dependence of the indirect band gap of isotopically purified ^{28}Si:P in the regime from 0.1 K to 3 K by high-resolution absorption spectroscopy of the donor bound exciton transition. The measurements increase the up-to-date precision of the temperature-dependent band gap change by more than one order of magnitude and reveal a T^{4} dependence which is about a factor of two less than observed in previous measurements. Such a T^{4} dependence is predicted by theory, but the absolute values differ between our experiment and the most up-to-date calculations by a factor of 30, corroborating that the electron-phonon interaction at low temperatures is still not correctly included into theory. What is more, the ability of such very high-precision band-gap measurements facilitates the use of time- and spatially resolved ^{28}Si:P absorption as a contactless, local thermometer and electric field sensor with a demonstrated time resolution of milliseconds.
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spelling doaj.art-58e00cdd28c54d598f36d187e6cec1cd2024-04-12T17:29:16ZengAmerican Physical SocietyPhysical Review Research2643-15642023-03-015101318210.1103/PhysRevResearch.5.013182Temperature dependence of the band gap of ^{28}Si:P at very low temperatures measured via time-resolved optical spectroscopyE. SauterN. V. AbrosimovJ. HübnerM. OestreichWe measure the temperature dependence of the indirect band gap of isotopically purified ^{28}Si:P in the regime from 0.1 K to 3 K by high-resolution absorption spectroscopy of the donor bound exciton transition. The measurements increase the up-to-date precision of the temperature-dependent band gap change by more than one order of magnitude and reveal a T^{4} dependence which is about a factor of two less than observed in previous measurements. Such a T^{4} dependence is predicted by theory, but the absolute values differ between our experiment and the most up-to-date calculations by a factor of 30, corroborating that the electron-phonon interaction at low temperatures is still not correctly included into theory. What is more, the ability of such very high-precision band-gap measurements facilitates the use of time- and spatially resolved ^{28}Si:P absorption as a contactless, local thermometer and electric field sensor with a demonstrated time resolution of milliseconds.http://doi.org/10.1103/PhysRevResearch.5.013182
spellingShingle E. Sauter
N. V. Abrosimov
J. Hübner
M. Oestreich
Temperature dependence of the band gap of ^{28}Si:P at very low temperatures measured via time-resolved optical spectroscopy
Physical Review Research
title Temperature dependence of the band gap of ^{28}Si:P at very low temperatures measured via time-resolved optical spectroscopy
title_full Temperature dependence of the band gap of ^{28}Si:P at very low temperatures measured via time-resolved optical spectroscopy
title_fullStr Temperature dependence of the band gap of ^{28}Si:P at very low temperatures measured via time-resolved optical spectroscopy
title_full_unstemmed Temperature dependence of the band gap of ^{28}Si:P at very low temperatures measured via time-resolved optical spectroscopy
title_short Temperature dependence of the band gap of ^{28}Si:P at very low temperatures measured via time-resolved optical spectroscopy
title_sort temperature dependence of the band gap of 28 si p at very low temperatures measured via time resolved optical spectroscopy
url http://doi.org/10.1103/PhysRevResearch.5.013182
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