Giant Seebeck effect across the field-induced metal-insulator transition of InAs

Abstract Lightly doped III–V semiconductor InAs is a dilute metal, which can be pushed beyond its extreme quantum limit upon the application of a modest magnetic field. In this regime, a Mott-Anderson metal–insulator transition, triggered by the magnetic field, leads to a depletion of carrier concen...

Full description

Bibliographic Details
Main Authors: Alexandre Jaoui, Gabriel Seyfarth, Carl Willem Rischau, Steffen Wiedmann, Siham Benhabib, Cyril Proust, Kamran Behnia, Benoît Fauqué
Format: Article
Language:English
Published: Nature Portfolio 2020-12-01
Series:npj Quantum Materials
Online Access:https://doi.org/10.1038/s41535-020-00296-0
_version_ 1818978959229976576
author Alexandre Jaoui
Gabriel Seyfarth
Carl Willem Rischau
Steffen Wiedmann
Siham Benhabib
Cyril Proust
Kamran Behnia
Benoît Fauqué
author_facet Alexandre Jaoui
Gabriel Seyfarth
Carl Willem Rischau
Steffen Wiedmann
Siham Benhabib
Cyril Proust
Kamran Behnia
Benoît Fauqué
author_sort Alexandre Jaoui
collection DOAJ
description Abstract Lightly doped III–V semiconductor InAs is a dilute metal, which can be pushed beyond its extreme quantum limit upon the application of a modest magnetic field. In this regime, a Mott-Anderson metal–insulator transition, triggered by the magnetic field, leads to a depletion of carrier concentration by more than one order of magnitude. Here, we show that this transition is accompanied by a 200-fold enhancement of the Seebeck coefficient, which becomes as large as 11.3 mV K−1 $$\approx 130\frac{{k}_{B}}{e}$$ ≈ 130 k B e at T = 8 K and B = 29 T. We find that the magnitude of this signal depends on sample dimensions and conclude that it is caused by phonon drag, resulting from a large difference between the scattering time of phonons (which are almost ballistic) and electrons (which are almost localized in the insulating state). Our results reveal a path to distinguish between possible sources of large thermoelectric response in other low-density systems pushed beyond the quantum limit.
first_indexed 2024-12-20T16:51:55Z
format Article
id doaj.art-5a18d7ae74a14aeab76deba7e45838a9
institution Directory Open Access Journal
issn 2397-4648
language English
last_indexed 2024-12-20T16:51:55Z
publishDate 2020-12-01
publisher Nature Portfolio
record_format Article
series npj Quantum Materials
spelling doaj.art-5a18d7ae74a14aeab76deba7e45838a92022-12-21T19:32:48ZengNature Portfolionpj Quantum Materials2397-46482020-12-01511610.1038/s41535-020-00296-0Giant Seebeck effect across the field-induced metal-insulator transition of InAsAlexandre Jaoui0Gabriel Seyfarth1Carl Willem Rischau2Steffen Wiedmann3Siham Benhabib4Cyril Proust5Kamran Behnia6Benoît Fauqué7JEIP, USR 3573 CNRS, Collège de France, PSL Research UniversityLaboratoire National des Champs Magnétiques Intenses (LNCMI-EMFL), CNRS, UGA, UPS, INSALaboratoire de Physique et Etude des Matériaux (CNRS/UPMC), Ecole Supérieure de Physique et de Chimie IndustriellesHigh Field Magnet Laboratory (HFML-EMFL), Radboud UniversityLaboratoire National des Champs Magnétiques Intenses (LNCMI-EMFL), CNRS, UGA, UPS, INSALaboratoire National des Champs Magnétiques Intenses (LNCMI-EMFL), CNRS, UGA, UPS, INSALaboratoire de Physique et Etude des Matériaux (CNRS/UPMC), Ecole Supérieure de Physique et de Chimie IndustriellesJEIP, USR 3573 CNRS, Collège de France, PSL Research UniversityAbstract Lightly doped III–V semiconductor InAs is a dilute metal, which can be pushed beyond its extreme quantum limit upon the application of a modest magnetic field. In this regime, a Mott-Anderson metal–insulator transition, triggered by the magnetic field, leads to a depletion of carrier concentration by more than one order of magnitude. Here, we show that this transition is accompanied by a 200-fold enhancement of the Seebeck coefficient, which becomes as large as 11.3 mV K−1 $$\approx 130\frac{{k}_{B}}{e}$$ ≈ 130 k B e at T = 8 K and B = 29 T. We find that the magnitude of this signal depends on sample dimensions and conclude that it is caused by phonon drag, resulting from a large difference between the scattering time of phonons (which are almost ballistic) and electrons (which are almost localized in the insulating state). Our results reveal a path to distinguish between possible sources of large thermoelectric response in other low-density systems pushed beyond the quantum limit.https://doi.org/10.1038/s41535-020-00296-0
spellingShingle Alexandre Jaoui
Gabriel Seyfarth
Carl Willem Rischau
Steffen Wiedmann
Siham Benhabib
Cyril Proust
Kamran Behnia
Benoît Fauqué
Giant Seebeck effect across the field-induced metal-insulator transition of InAs
npj Quantum Materials
title Giant Seebeck effect across the field-induced metal-insulator transition of InAs
title_full Giant Seebeck effect across the field-induced metal-insulator transition of InAs
title_fullStr Giant Seebeck effect across the field-induced metal-insulator transition of InAs
title_full_unstemmed Giant Seebeck effect across the field-induced metal-insulator transition of InAs
title_short Giant Seebeck effect across the field-induced metal-insulator transition of InAs
title_sort giant seebeck effect across the field induced metal insulator transition of inas
url https://doi.org/10.1038/s41535-020-00296-0
work_keys_str_mv AT alexandrejaoui giantseebeckeffectacrossthefieldinducedmetalinsulatortransitionofinas
AT gabrielseyfarth giantseebeckeffectacrossthefieldinducedmetalinsulatortransitionofinas
AT carlwillemrischau giantseebeckeffectacrossthefieldinducedmetalinsulatortransitionofinas
AT steffenwiedmann giantseebeckeffectacrossthefieldinducedmetalinsulatortransitionofinas
AT sihambenhabib giantseebeckeffectacrossthefieldinducedmetalinsulatortransitionofinas
AT cyrilproust giantseebeckeffectacrossthefieldinducedmetalinsulatortransitionofinas
AT kamranbehnia giantseebeckeffectacrossthefieldinducedmetalinsulatortransitionofinas
AT benoitfauque giantseebeckeffectacrossthefieldinducedmetalinsulatortransitionofinas