In Situ Study of the Impact of Aberration-Corrected Electron-Beam Lithography on the Electronic Transport of Suspended Graphene Devices

The implementation of aberration-corrected electron beam lithography (AC-EBL) in a 200 keV scanning transmission electron microscope (STEM) is a novel technique that could be used for the fabrication of quantum devices based on 2D atomic crystals with single nanometer critical dimensions, allowing t...

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Main Authors: Naomi Mizuno, Fernando Camino, Xu Du
Format: Article
Language:English
Published: MDPI AG 2020-04-01
Series:Nanomaterials
Subjects:
Online Access:https://www.mdpi.com/2079-4991/10/4/666
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author Naomi Mizuno
Fernando Camino
Xu Du
author_facet Naomi Mizuno
Fernando Camino
Xu Du
author_sort Naomi Mizuno
collection DOAJ
description The implementation of aberration-corrected electron beam lithography (AC-EBL) in a 200 keV scanning transmission electron microscope (STEM) is a novel technique that could be used for the fabrication of quantum devices based on 2D atomic crystals with single nanometer critical dimensions, allowing to observe more robust quantum effects. In this work we study electron beam sculpturing of nanostructures on suspended graphene field effect transistors using AC-EBL, focusing on the in situ characterization of the impact of electron beam exposure on device electronic transport quality. When AC-EBL is performed on a graphene channel (local exposure) or on the outside vicinity of a graphene channel (non-local exposure), the charge transport characteristics of graphene can be significantly affected due to charge doping and scattering. While the detrimental effect of non-local exposure can be largely removed by vigorous annealing, local-exposure induced damage is irreversible and cannot be fixed by annealing. We discuss the possible causes of the observed exposure effects. Our results provide guidance to the future development of high-energy electron beam lithography for nanomaterial device fabrication.
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spelling doaj.art-78963cfdc92f4669a400185ae75c2c6c2023-11-19T20:30:45ZengMDPI AGNanomaterials2079-49912020-04-0110466610.3390/nano10040666In Situ Study of the Impact of Aberration-Corrected Electron-Beam Lithography on the Electronic Transport of Suspended Graphene DevicesNaomi Mizuno0Fernando Camino1Xu Du2Department of Physics and Astronomy, Stony Brook University, Stony Brook, NY 11794-3800, USACenter for Functional Nanomaterials, Brookhaven National Laboratory, Upton, NY 11973, USADepartment of Physics and Astronomy, Stony Brook University, Stony Brook, NY 11794-3800, USAThe implementation of aberration-corrected electron beam lithography (AC-EBL) in a 200 keV scanning transmission electron microscope (STEM) is a novel technique that could be used for the fabrication of quantum devices based on 2D atomic crystals with single nanometer critical dimensions, allowing to observe more robust quantum effects. In this work we study electron beam sculpturing of nanostructures on suspended graphene field effect transistors using AC-EBL, focusing on the in situ characterization of the impact of electron beam exposure on device electronic transport quality. When AC-EBL is performed on a graphene channel (local exposure) or on the outside vicinity of a graphene channel (non-local exposure), the charge transport characteristics of graphene can be significantly affected due to charge doping and scattering. While the detrimental effect of non-local exposure can be largely removed by vigorous annealing, local-exposure induced damage is irreversible and cannot be fixed by annealing. We discuss the possible causes of the observed exposure effects. Our results provide guidance to the future development of high-energy electron beam lithography for nanomaterial device fabrication.https://www.mdpi.com/2079-4991/10/4/666graphene devicese-beam damagee-beam lithographyaberration corrected
spellingShingle Naomi Mizuno
Fernando Camino
Xu Du
In Situ Study of the Impact of Aberration-Corrected Electron-Beam Lithography on the Electronic Transport of Suspended Graphene Devices
Nanomaterials
graphene devices
e-beam damage
e-beam lithography
aberration corrected
title In Situ Study of the Impact of Aberration-Corrected Electron-Beam Lithography on the Electronic Transport of Suspended Graphene Devices
title_full In Situ Study of the Impact of Aberration-Corrected Electron-Beam Lithography on the Electronic Transport of Suspended Graphene Devices
title_fullStr In Situ Study of the Impact of Aberration-Corrected Electron-Beam Lithography on the Electronic Transport of Suspended Graphene Devices
title_full_unstemmed In Situ Study of the Impact of Aberration-Corrected Electron-Beam Lithography on the Electronic Transport of Suspended Graphene Devices
title_short In Situ Study of the Impact of Aberration-Corrected Electron-Beam Lithography on the Electronic Transport of Suspended Graphene Devices
title_sort in situ study of the impact of aberration corrected electron beam lithography on the electronic transport of suspended graphene devices
topic graphene devices
e-beam damage
e-beam lithography
aberration corrected
url https://www.mdpi.com/2079-4991/10/4/666
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