Second-order spectral lineshapes from charged interfaces

Charged interfaces are important in chemical systems, but the influence of charge on vibrational sum frequency spectra has only recently been considered. Here the authors show the importance of accounting for the interfacial potential-dependent χ(3) term in interpreting spectral lineshapes from char...

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Bibliographic Details
Main Authors: Paul E. Ohno, Hong-fei Wang, Franz M. Geiger
Format: Article
Language:English
Published: Nature Portfolio 2017-10-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-017-01088-0