Second-order spectral lineshapes from charged interfaces

Charged interfaces are important in chemical systems, but the influence of charge on vibrational sum frequency spectra has only recently been considered. Here the authors show the importance of accounting for the interfacial potential-dependent χ(3) term in interpreting spectral lineshapes from char...

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Main Authors: Paul E. Ohno, Hong-fei Wang, Franz M. Geiger
Format: Article
Language:English
Published: Nature Portfolio 2017-10-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-017-01088-0
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author Paul E. Ohno
Hong-fei Wang
Franz M. Geiger
author_facet Paul E. Ohno
Hong-fei Wang
Franz M. Geiger
author_sort Paul E. Ohno
collection DOAJ
description Charged interfaces are important in chemical systems, but the influence of charge on vibrational sum frequency spectra has only recently been considered. Here the authors show the importance of accounting for the interfacial potential-dependent χ(3) term in interpreting spectral lineshapes from charged interfaces.
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spelling doaj.art-7b1cc2d9b1a14b74b4692aeeefb71f222022-12-21T20:31:29ZengNature PortfolioNature Communications2041-17232017-10-01811910.1038/s41467-017-01088-0Second-order spectral lineshapes from charged interfacesPaul E. Ohno0Hong-fei Wang1Franz M. Geiger2Department of Chemistry, Northwestern UniversityDepartment of Chemistry and Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Fudan UniversityDepartment of Chemistry, Northwestern UniversityCharged interfaces are important in chemical systems, but the influence of charge on vibrational sum frequency spectra has only recently been considered. Here the authors show the importance of accounting for the interfacial potential-dependent χ(3) term in interpreting spectral lineshapes from charged interfaces.https://doi.org/10.1038/s41467-017-01088-0
spellingShingle Paul E. Ohno
Hong-fei Wang
Franz M. Geiger
Second-order spectral lineshapes from charged interfaces
Nature Communications
title Second-order spectral lineshapes from charged interfaces
title_full Second-order spectral lineshapes from charged interfaces
title_fullStr Second-order spectral lineshapes from charged interfaces
title_full_unstemmed Second-order spectral lineshapes from charged interfaces
title_short Second-order spectral lineshapes from charged interfaces
title_sort second order spectral lineshapes from charged interfaces
url https://doi.org/10.1038/s41467-017-01088-0
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AT hongfeiwang secondorderspectrallineshapesfromchargedinterfaces
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