Second-order spectral lineshapes from charged interfaces
Charged interfaces are important in chemical systems, but the influence of charge on vibrational sum frequency spectra has only recently been considered. Here the authors show the importance of accounting for the interfacial potential-dependent χ(3) term in interpreting spectral lineshapes from char...
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Format: | Article |
Language: | English |
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Nature Portfolio
2017-10-01
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Series: | Nature Communications |
Online Access: | https://doi.org/10.1038/s41467-017-01088-0 |
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author | Paul E. Ohno Hong-fei Wang Franz M. Geiger |
author_facet | Paul E. Ohno Hong-fei Wang Franz M. Geiger |
author_sort | Paul E. Ohno |
collection | DOAJ |
description | Charged interfaces are important in chemical systems, but the influence of charge on vibrational sum frequency spectra has only recently been considered. Here the authors show the importance of accounting for the interfacial potential-dependent χ(3) term in interpreting spectral lineshapes from charged interfaces. |
first_indexed | 2024-12-19T06:57:39Z |
format | Article |
id | doaj.art-7b1cc2d9b1a14b74b4692aeeefb71f22 |
institution | Directory Open Access Journal |
issn | 2041-1723 |
language | English |
last_indexed | 2024-12-19T06:57:39Z |
publishDate | 2017-10-01 |
publisher | Nature Portfolio |
record_format | Article |
series | Nature Communications |
spelling | doaj.art-7b1cc2d9b1a14b74b4692aeeefb71f222022-12-21T20:31:29ZengNature PortfolioNature Communications2041-17232017-10-01811910.1038/s41467-017-01088-0Second-order spectral lineshapes from charged interfacesPaul E. Ohno0Hong-fei Wang1Franz M. Geiger2Department of Chemistry, Northwestern UniversityDepartment of Chemistry and Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Fudan UniversityDepartment of Chemistry, Northwestern UniversityCharged interfaces are important in chemical systems, but the influence of charge on vibrational sum frequency spectra has only recently been considered. Here the authors show the importance of accounting for the interfacial potential-dependent χ(3) term in interpreting spectral lineshapes from charged interfaces.https://doi.org/10.1038/s41467-017-01088-0 |
spellingShingle | Paul E. Ohno Hong-fei Wang Franz M. Geiger Second-order spectral lineshapes from charged interfaces Nature Communications |
title | Second-order spectral lineshapes from charged interfaces |
title_full | Second-order spectral lineshapes from charged interfaces |
title_fullStr | Second-order spectral lineshapes from charged interfaces |
title_full_unstemmed | Second-order spectral lineshapes from charged interfaces |
title_short | Second-order spectral lineshapes from charged interfaces |
title_sort | second order spectral lineshapes from charged interfaces |
url | https://doi.org/10.1038/s41467-017-01088-0 |
work_keys_str_mv | AT pauleohno secondorderspectrallineshapesfromchargedinterfaces AT hongfeiwang secondorderspectrallineshapesfromchargedinterfaces AT franzmgeiger secondorderspectrallineshapesfromchargedinterfaces |