Triplet-mediated spin entanglement between organic radicals: integrating first principles and open-quantum-system simulations

Abstract Controlling molecular spin quantum bits optically offers the potential to effectively reduce decoherence and raise the working temperature of quantum computers. Here, exchange interactions and spin dynamics, as mediated by an optically driven triplet state, are calculated for a molecule tha...

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Bibliographic Details
Main Authors: Tianhong Huang, Jiawei Chang, Lin Ma, Andrew J. Fisher, Nicholas M. Harrison, Taoyu Zou, Hai Wang, Wei Wu
Format: Article
Language:English
Published: Nature Portfolio 2023-12-01
Series:NPG Asia Materials
Online Access:https://doi.org/10.1038/s41427-023-00510-y