Probing the limits of optical cycling in a predissociative diatomic molecule
Molecular predissociation, the spontaneous nonradiative bond-breaking process, can limit the ability to scatter a large number of photons required to reach the ultracold regime in laser cooling. Unlike rovibrational branching, predissociation is irreversible since the fragments fly apart with high k...
Main Authors: | , , , , , , , , |
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Format: | Article |
Language: | English |
Published: |
American Physical Society
2023-10-01
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Series: | Physical Review Research |
Online Access: | http://doi.org/10.1103/PhysRevResearch.5.043070 |