Probing the limits of optical cycling in a predissociative diatomic molecule

Molecular predissociation, the spontaneous nonradiative bond-breaking process, can limit the ability to scatter a large number of photons required to reach the ultracold regime in laser cooling. Unlike rovibrational branching, predissociation is irreversible since the fragments fly apart with high k...

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Bibliographic Details
Main Authors: Qi Sun, Claire E. Dickerson, Jinyu Dai, Isaac M. Pope, Lan Cheng, Daniel Neuhauser, Anastassia N. Alexandrova, Debayan Mitra, Tanya Zelevinsky
Format: Article
Language:English
Published: American Physical Society 2023-10-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.5.043070