Contribution to Excitonic Linewidth from Free Carrier–Exciton Scattering in Layered Materials: The Example of hBN

Scattering of excitons by free carriers is a phenomenon, which is especially important when considering moderately to heavily doped semiconductors in low-temperature experiments, where the interaction of excitons with acoustic and optical phonons is reduced. In this paper, we consider the scattering...

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Main Authors: Maurício F. C. Martins Quintela, Nuno M. R. Peres
Format: Article
Language:English
Published: MDPI AG 2022-08-01
Series:Applied Sciences
Subjects:
Online Access:https://www.mdpi.com/2076-3417/12/15/7872
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author Maurício F. C. Martins Quintela
Nuno M. R. Peres
author_facet Maurício F. C. Martins Quintela
Nuno M. R. Peres
author_sort Maurício F. C. Martins Quintela
collection DOAJ
description Scattering of excitons by free carriers is a phenomenon, which is especially important when considering moderately to heavily doped semiconductors in low-temperature experiments, where the interaction of excitons with acoustic and optical phonons is reduced. In this paper, we consider the scattering of excitons by free carriers in monolayer hexagonal boron nitride encapsulated by a dielectric medium. We describe the excitonic states by variational wave functions, modeling the electrostatic interaction via the Rytova–Keldysh potential. Making the distinction between elastic and inelastic scattering, the relevance of each transition between excitonic states is also considered. Finally, we discuss the contribution of free carrier scattering to the excitonic linewidth, analyzing both its temperature and carrier density dependence.
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spelling doaj.art-83d390b235334b6b9039f96e3dc4f2be2023-11-30T22:11:59ZengMDPI AGApplied Sciences2076-34172022-08-011215787210.3390/app12157872Contribution to Excitonic Linewidth from Free Carrier–Exciton Scattering in Layered Materials: The Example of hBNMaurício F. C. Martins Quintela0Nuno M. R. Peres1Department of Physics, Physics Center of Minho, Campus of Gualtar, Porto Universities (CF–UM–UP), 4710-057 Braga, PortugalDepartment of Physics, Physics Center of Minho, Campus of Gualtar, Porto Universities (CF–UM–UP), 4710-057 Braga, PortugalScattering of excitons by free carriers is a phenomenon, which is especially important when considering moderately to heavily doped semiconductors in low-temperature experiments, where the interaction of excitons with acoustic and optical phonons is reduced. In this paper, we consider the scattering of excitons by free carriers in monolayer hexagonal boron nitride encapsulated by a dielectric medium. We describe the excitonic states by variational wave functions, modeling the electrostatic interaction via the Rytova–Keldysh potential. Making the distinction between elastic and inelastic scattering, the relevance of each transition between excitonic states is also considered. Finally, we discuss the contribution of free carrier scattering to the excitonic linewidth, analyzing both its temperature and carrier density dependence.https://www.mdpi.com/2076-3417/12/15/7872excitonlinewidthfree carriermonolayerscatteringtemperature
spellingShingle Maurício F. C. Martins Quintela
Nuno M. R. Peres
Contribution to Excitonic Linewidth from Free Carrier–Exciton Scattering in Layered Materials: The Example of hBN
Applied Sciences
exciton
linewidth
free carrier
monolayer
scattering
temperature
title Contribution to Excitonic Linewidth from Free Carrier–Exciton Scattering in Layered Materials: The Example of hBN
title_full Contribution to Excitonic Linewidth from Free Carrier–Exciton Scattering in Layered Materials: The Example of hBN
title_fullStr Contribution to Excitonic Linewidth from Free Carrier–Exciton Scattering in Layered Materials: The Example of hBN
title_full_unstemmed Contribution to Excitonic Linewidth from Free Carrier–Exciton Scattering in Layered Materials: The Example of hBN
title_short Contribution to Excitonic Linewidth from Free Carrier–Exciton Scattering in Layered Materials: The Example of hBN
title_sort contribution to excitonic linewidth from free carrier exciton scattering in layered materials the example of hbn
topic exciton
linewidth
free carrier
monolayer
scattering
temperature
url https://www.mdpi.com/2076-3417/12/15/7872
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