Vibronic Relaxation Pathways in Molecular Spin Qubit Na<sub>9</sub>[Ho(W<sub>5</sub>O<sub>18</sub>)<sub>2</sub>]·35H<sub>2</sub>O under Pressure

Vibronic Relaxation Pathways in Molecular Spin Qubit Na<sub>9</sub>[Ho(W<sub>5</sub>O<sub>18</sub>)<sub>2</sub>]·35H<sub>2</sub>O under Pressure

In order to explore how spectral sparsity and vibronic decoherence pathways can be controlled in a model qubit system with atomic clock transitions, we combined diamond anvil cell techniques with synchrotron-based far infrared spectroscopy and first-principles calculations to reveal the vibrational...

Full description

Bibliographic Details
Main Authors: Janice L. Musfeldt, Zhenxian Liu, Diego López-Alcalá, Yan Duan, Alejandro Gaita-Ariño, José J. Baldoví, Eugenio Coronado
Format: Article
Language:English
Published: MDPI AG 2023-02-01
Series:Magnetochemistry
Subjects:
spin qubit
vibronic coupling
strategies to minimize decoherence
high pressure vibrational spectroscopy
Online Access:https://www.mdpi.com/2312-7481/9/2/53

Internet

https://www.mdpi.com/2312-7481/9/2/53

Similar Items