Resonance Raman optical cycling for high-fidelity fluorescence detection of molecules

We propose and demonstrate a technique that combines Raman scattering and optical cycling in molecules with diagonal Franck-Condon factors. This resonance Raman optical cycling manipulates molecules to behave like efficient fluorophores, with discrete absorption and emission profiles that are readil...

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Bibliographic Details
Main Authors: J. C. Shaw, J. C. Schnaubelt, D. J. McCarron
Format: Article
Language:English
Published: American Physical Society 2021-12-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.3.L042041