Entangled Biphoton Enhanced Double Quantum Coherence Signal as a Probe for Cavity Polariton Correlations in Presence of Phonon Induced Dephasing

We theoretically propose a biphoton entanglement-enhanced multidimensional spectroscopic technique as a probe for the dissipative polariton dynamics in the ultrafast regime. It is applied to the cavity-confined monomeric photosynthetic complex that represents a prototypical multi-site excitonic quan...

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Bibliographic Details
Main Authors: Arunangshu Debnath, Angel Rubio
Format: Article
Language:English
Published: Frontiers Media S.A. 2022-07-01
Series:Frontiers in Physics
Subjects:
Online Access:https://www.frontiersin.org/articles/10.3389/fphy.2022.879113/full