InGaN as a Substrate for AC Photoelectrochemical Imaging

AC photoelectrochemical imaging at electrolyte−semiconductor interfaces provides spatially resolved information such as surface potentials, ion concentrations and electrical impedance. In this work, thin films of InGaN/GaN were used successfully for AC photoelectrochemical imaging, and exp...

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Main Authors: Bo Zhou, Anirban Das, Menno J. Kappers, Rachel A. Oliver, Colin J. Humphreys, Steffi Krause
Format: Article
Language:English
Published: MDPI AG 2019-10-01
Series:Sensors
Subjects:
Online Access:https://www.mdpi.com/1424-8220/19/20/4386
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author Bo Zhou
Anirban Das
Menno J. Kappers
Rachel A. Oliver
Colin J. Humphreys
Steffi Krause
author_facet Bo Zhou
Anirban Das
Menno J. Kappers
Rachel A. Oliver
Colin J. Humphreys
Steffi Krause
author_sort Bo Zhou
collection DOAJ
description AC photoelectrochemical imaging at electrolyte−semiconductor interfaces provides spatially resolved information such as surface potentials, ion concentrations and electrical impedance. In this work, thin films of InGaN/GaN were used successfully for AC photoelectrochemical imaging, and experimentally shown to generate a considerable photocurrent under illumination with a 405 nm modulated diode laser at comparatively high frequencies and low applied DC potentials, making this a promising substrate for bioimaging applications. Linear sweep voltammetry showed negligible dark currents. The imaging capabilities of the sensor substrate were demonstrated with a model system and showed a lateral resolution of 7 microns.
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spelling doaj.art-9c13b59d436040e5ada0c300f0b845c52022-12-22T04:27:19ZengMDPI AGSensors1424-82202019-10-011920438610.3390/s19204386s19204386InGaN as a Substrate for AC Photoelectrochemical ImagingBo Zhou0Anirban Das1Menno J. Kappers2Rachel A. Oliver3Colin J. Humphreys4Steffi Krause5School of Engineering and Materials Science, Queen Mary University of London, Mile End Road, London E1 4NS, UKSchool of Engineering and Materials Science, Queen Mary University of London, Mile End Road, London E1 4NS, UKDepartment of Materials Science and Metallurgy, University of Cambridge, 27 Charles Babbage Road, Cambridge CB3 0FS, UKDepartment of Materials Science and Metallurgy, University of Cambridge, 27 Charles Babbage Road, Cambridge CB3 0FS, UKSchool of Engineering and Materials Science, Queen Mary University of London, Mile End Road, London E1 4NS, UKSchool of Engineering and Materials Science, Queen Mary University of London, Mile End Road, London E1 4NS, UKAC photoelectrochemical imaging at electrolyte−semiconductor interfaces provides spatially resolved information such as surface potentials, ion concentrations and electrical impedance. In this work, thin films of InGaN/GaN were used successfully for AC photoelectrochemical imaging, and experimentally shown to generate a considerable photocurrent under illumination with a 405 nm modulated diode laser at comparatively high frequencies and low applied DC potentials, making this a promising substrate for bioimaging applications. Linear sweep voltammetry showed negligible dark currents. The imaging capabilities of the sensor substrate were demonstrated with a model system and showed a lateral resolution of 7 microns.https://www.mdpi.com/1424-8220/19/20/4386photoelectrochemistryingan/gan epilayercell imaginglight-activated electrochemistrylight-addressable potentiometric sensor
spellingShingle Bo Zhou
Anirban Das
Menno J. Kappers
Rachel A. Oliver
Colin J. Humphreys
Steffi Krause
InGaN as a Substrate for AC Photoelectrochemical Imaging
Sensors
photoelectrochemistry
ingan/gan epilayer
cell imaging
light-activated electrochemistry
light-addressable potentiometric sensor
title InGaN as a Substrate for AC Photoelectrochemical Imaging
title_full InGaN as a Substrate for AC Photoelectrochemical Imaging
title_fullStr InGaN as a Substrate for AC Photoelectrochemical Imaging
title_full_unstemmed InGaN as a Substrate for AC Photoelectrochemical Imaging
title_short InGaN as a Substrate for AC Photoelectrochemical Imaging
title_sort ingan as a substrate for ac photoelectrochemical imaging
topic photoelectrochemistry
ingan/gan epilayer
cell imaging
light-activated electrochemistry
light-addressable potentiometric sensor
url https://www.mdpi.com/1424-8220/19/20/4386
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