Particulate reduction in ternary-compound film growth via pulsed laser deposition from segmented binary-targets

We present the hetero-epitaxial growth of high-quality crystalline Y _3 Ga _5 O _12 onto a 〈100〉-oriented YAG substrate via pulsed laser deposition, using mixed ternary-compound and segmented binary-compound targets. We observe that a Y _3 Ga _5 O _12 film fabricated using a segmented target (Y _2 O...

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Main Authors: James A Grant-Jacob, Jake J Prentice, Stephen J Beecher, David P Shepherd, Robert W Eason, Jacob I Mackenzie
Format: Article
Language:English
Published: IOP Publishing 2018-01-01
Series:Materials Research Express
Subjects:
Online Access:https://doi.org/10.1088/2053-1591/aab0ef
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author James A Grant-Jacob
Jake J Prentice
Stephen J Beecher
David P Shepherd
Robert W Eason
Jacob I Mackenzie
author_facet James A Grant-Jacob
Jake J Prentice
Stephen J Beecher
David P Shepherd
Robert W Eason
Jacob I Mackenzie
author_sort James A Grant-Jacob
collection DOAJ
description We present the hetero-epitaxial growth of high-quality crystalline Y _3 Ga _5 O _12 onto a 〈100〉-oriented YAG substrate via pulsed laser deposition, using mixed ternary-compound and segmented binary-compound targets. We observe that a Y _3 Ga _5 O _12 film fabricated using a segmented target (Y _2 O _3 /Ga _2 O _3 ) contained ∼100 times fewer scattering points than a film grown using a mixed Y _3 Ga _5 O _12 target. We show that following ablation, the surface of the mixed compound (ternary) target had laser-induced cone structures, whereas the surface of single compound (binary) targets did not. It is concluded that the different ablation dynamics of the oxide constituents in the respective targets plays a significant role in the origin of the scattering points in the resultant films.
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spelling doaj.art-aa5328d8acf34d798b682bf5a467c2702023-08-09T15:21:36ZengIOP PublishingMaterials Research Express2053-15912018-01-015303640210.1088/2053-1591/aab0efParticulate reduction in ternary-compound film growth via pulsed laser deposition from segmented binary-targetsJames A Grant-Jacob0https://orcid.org/0000-0002-4270-4247Jake J Prentice1Stephen J Beecher2David P Shepherd3Robert W Eason4Jacob I Mackenzie5Optoelectronics Research Centre, University of Southampton , Southampton, SO17 1BJ, United KingdomOptoelectronics Research Centre, University of Southampton , Southampton, SO17 1BJ, United KingdomOptoelectronics Research Centre, University of Southampton , Southampton, SO17 1BJ, United KingdomOptoelectronics Research Centre, University of Southampton , Southampton, SO17 1BJ, United KingdomOptoelectronics Research Centre, University of Southampton , Southampton, SO17 1BJ, United KingdomOptoelectronics Research Centre, University of Southampton , Southampton, SO17 1BJ, United KingdomWe present the hetero-epitaxial growth of high-quality crystalline Y _3 Ga _5 O _12 onto a 〈100〉-oriented YAG substrate via pulsed laser deposition, using mixed ternary-compound and segmented binary-compound targets. We observe that a Y _3 Ga _5 O _12 film fabricated using a segmented target (Y _2 O _3 /Ga _2 O _3 ) contained ∼100 times fewer scattering points than a film grown using a mixed Y _3 Ga _5 O _12 target. We show that following ablation, the surface of the mixed compound (ternary) target had laser-induced cone structures, whereas the surface of single compound (binary) targets did not. It is concluded that the different ablation dynamics of the oxide constituents in the respective targets plays a significant role in the origin of the scattering points in the resultant films.https://doi.org/10.1088/2053-1591/aab0efpulsed laser depositioncrystal structuresurface structurethin filmsceramic target81.15.Fg
spellingShingle James A Grant-Jacob
Jake J Prentice
Stephen J Beecher
David P Shepherd
Robert W Eason
Jacob I Mackenzie
Particulate reduction in ternary-compound film growth via pulsed laser deposition from segmented binary-targets
Materials Research Express
pulsed laser deposition
crystal structure
surface structure
thin films
ceramic target
81.15.Fg
title Particulate reduction in ternary-compound film growth via pulsed laser deposition from segmented binary-targets
title_full Particulate reduction in ternary-compound film growth via pulsed laser deposition from segmented binary-targets
title_fullStr Particulate reduction in ternary-compound film growth via pulsed laser deposition from segmented binary-targets
title_full_unstemmed Particulate reduction in ternary-compound film growth via pulsed laser deposition from segmented binary-targets
title_short Particulate reduction in ternary-compound film growth via pulsed laser deposition from segmented binary-targets
title_sort particulate reduction in ternary compound film growth via pulsed laser deposition from segmented binary targets
topic pulsed laser deposition
crystal structure
surface structure
thin films
ceramic target
81.15.Fg
url https://doi.org/10.1088/2053-1591/aab0ef
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