Essential Role of Triplet Diradical Character for Large Magnetoresistance in Quinoidal Organic Semiconductor with High Electron Mobility

Abstract A diradicaloid molecule with high semiconducting performance is synthesized based on the quinoidal benzo[1,2‐b:4,5‐b′]dithiophene structure. The diradical character is investigated by quantum chemical calculations and variable temperature electron spin resonance. The diode devices based on...

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Bibliographic Details
Main Authors: Chao Wang, Hua Hao, Keisuke Tajima
Format: Article
Language:English
Published: Wiley 2022-05-01
Series:Advanced Science
Subjects:
Online Access:https://doi.org/10.1002/advs.202201045