2D-GaN/AlN Multiple Quantum Disks/Quantum Well Heterostructures for High-Power Electron-Beam Pumped UVC Emitters

This article describes GaN/AlN heterostructures for ultraviolet-C (UVC) emitters with multiple (up to 400 periods) two-dimensional (2D)-quantum disk/quantum well structures with the same GaN nominal thicknesses of 1.5 and 16 ML-thick AlN barrier layers, which were grown by plasma-assisted molecular-...

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Main Authors: Valentin Jmerik, Dmitrii Nechaev, Alexey Semenov, Eugenii Evropeitsev, Tatiana Shubina, Alexey Toropov, Maria Yagovkina, Prokhor Alekseev, Bogdan Borodin, Kseniya Orekhova, Vladimir Kozlovsky, Mikhail Zverev, Nikita Gamov, Tao Wang, Xinqiang Wang, Markus Pristovsek, Hiroshi Amano, Sergey Ivanov
Format: Article
Language:English
Published: MDPI AG 2023-03-01
Series:Nanomaterials
Subjects:
Online Access:https://www.mdpi.com/2079-4991/13/6/1077
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author Valentin Jmerik
Dmitrii Nechaev
Alexey Semenov
Eugenii Evropeitsev
Tatiana Shubina
Alexey Toropov
Maria Yagovkina
Prokhor Alekseev
Bogdan Borodin
Kseniya Orekhova
Vladimir Kozlovsky
Mikhail Zverev
Nikita Gamov
Tao Wang
Xinqiang Wang
Markus Pristovsek
Hiroshi Amano
Sergey Ivanov
author_facet Valentin Jmerik
Dmitrii Nechaev
Alexey Semenov
Eugenii Evropeitsev
Tatiana Shubina
Alexey Toropov
Maria Yagovkina
Prokhor Alekseev
Bogdan Borodin
Kseniya Orekhova
Vladimir Kozlovsky
Mikhail Zverev
Nikita Gamov
Tao Wang
Xinqiang Wang
Markus Pristovsek
Hiroshi Amano
Sergey Ivanov
author_sort Valentin Jmerik
collection DOAJ
description This article describes GaN/AlN heterostructures for ultraviolet-C (UVC) emitters with multiple (up to 400 periods) two-dimensional (2D)-quantum disk/quantum well structures with the same GaN nominal thicknesses of 1.5 and 16 ML-thick AlN barrier layers, which were grown by plasma-assisted molecular-beam epitaxy in a wide range of gallium and activated nitrogen flux ratios (Ga/N<sub>2</sub>*) on <i>c</i>-sapphire substrates. An increase in the Ga/N<sub>2</sub>* ratio from 1.1 to 2.2 made it possible to change the 2D-topography of the structures due to a transition from the mixed spiral and 2D-nucleation growth to a purely spiral growth. As a result, the emission energy (wavelength) could be varied from 5.21 eV (238 nm) to 4.68 eV (265 nm) owing to the correspondingly increased carrier localization energy. Using electron-beam pumping with a maximum pulse current of 2 A at an electron energy of 12.5 keV, a maximum output optical power of 50 W was achieved for the 265 nm structure, while the structure emitting at 238 nm demonstrated a power of 10 W.
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spelling doaj.art-e68a391da1a54fb48871c3f2373bfe322023-11-17T13:01:15ZengMDPI AGNanomaterials2079-49912023-03-01136107710.3390/nano130610772D-GaN/AlN Multiple Quantum Disks/Quantum Well Heterostructures for High-Power Electron-Beam Pumped UVC EmittersValentin Jmerik0Dmitrii Nechaev1Alexey Semenov2Eugenii Evropeitsev3Tatiana Shubina4Alexey Toropov5Maria Yagovkina6Prokhor Alekseev7Bogdan Borodin8Kseniya Orekhova9Vladimir Kozlovsky10Mikhail Zverev11Nikita Gamov12Tao Wang13Xinqiang Wang14Markus Pristovsek15Hiroshi Amano16Sergey Ivanov17Ioffe Institute, 26 Politekhnicheskaya, Saint Petersburg 194021, RussiaIoffe Institute, 26 Politekhnicheskaya, Saint Petersburg 194021, RussiaIoffe Institute, 26 Politekhnicheskaya, Saint Petersburg 194021, RussiaIoffe Institute, 26 Politekhnicheskaya, Saint Petersburg 194021, RussiaIoffe Institute, 26 Politekhnicheskaya, Saint Petersburg 194021, RussiaIoffe Institute, 26 Politekhnicheskaya, Saint Petersburg 194021, RussiaIoffe Institute, 26 Politekhnicheskaya, Saint Petersburg 194021, RussiaIoffe Institute, 26 Politekhnicheskaya, Saint Petersburg 194021, RussiaIoffe Institute, 26 Politekhnicheskaya, Saint Petersburg 194021, RussiaIoffe Institute, 26 Politekhnicheskaya, Saint Petersburg 194021, RussiaLebedev Physical Institute, Leninsky Avenue 53, Moscow 119991, RussiaLebedev Physical Institute, Leninsky Avenue 53, Moscow 119991, RussiaLebedev Physical Institute, Leninsky Avenue 53, Moscow 119991, RussiaState Key Laboratory for Mesoscopic Physics and Frontiers Science Center for Nanooptoelectronics, School of Physics, Peking University, Beijing 100871, ChinaState Key Laboratory for Mesoscopic Physics and Frontiers Science Center for Nanooptoelectronics, School of Physics, Peking University, Beijing 100871, ChinaInstitute of Materials and Systems for Sustainability (IMaSS), Nagoya University, Chikusa-Ku, Furo-Cho, Nagoya 464-8601, JapanInstitute of Materials and Systems for Sustainability (IMaSS), Nagoya University, Chikusa-Ku, Furo-Cho, Nagoya 464-8601, JapanIoffe Institute, 26 Politekhnicheskaya, Saint Petersburg 194021, RussiaThis article describes GaN/AlN heterostructures for ultraviolet-C (UVC) emitters with multiple (up to 400 periods) two-dimensional (2D)-quantum disk/quantum well structures with the same GaN nominal thicknesses of 1.5 and 16 ML-thick AlN barrier layers, which were grown by plasma-assisted molecular-beam epitaxy in a wide range of gallium and activated nitrogen flux ratios (Ga/N<sub>2</sub>*) on <i>c</i>-sapphire substrates. An increase in the Ga/N<sub>2</sub>* ratio from 1.1 to 2.2 made it possible to change the 2D-topography of the structures due to a transition from the mixed spiral and 2D-nucleation growth to a purely spiral growth. As a result, the emission energy (wavelength) could be varied from 5.21 eV (238 nm) to 4.68 eV (265 nm) owing to the correspondingly increased carrier localization energy. Using electron-beam pumping with a maximum pulse current of 2 A at an electron energy of 12.5 keV, a maximum output optical power of 50 W was achieved for the 265 nm structure, while the structure emitting at 238 nm demonstrated a power of 10 W.https://www.mdpi.com/2079-4991/13/6/1077monolayer thick GaN/AlN multiple quantum wellsIII-nitridescarrier localizationplasma-assisted molecular beam epitaxyelectron-beam pumped UVC emitters
spellingShingle Valentin Jmerik
Dmitrii Nechaev
Alexey Semenov
Eugenii Evropeitsev
Tatiana Shubina
Alexey Toropov
Maria Yagovkina
Prokhor Alekseev
Bogdan Borodin
Kseniya Orekhova
Vladimir Kozlovsky
Mikhail Zverev
Nikita Gamov
Tao Wang
Xinqiang Wang
Markus Pristovsek
Hiroshi Amano
Sergey Ivanov
2D-GaN/AlN Multiple Quantum Disks/Quantum Well Heterostructures for High-Power Electron-Beam Pumped UVC Emitters
Nanomaterials
monolayer thick GaN/AlN multiple quantum wells
III-nitrides
carrier localization
plasma-assisted molecular beam epitaxy
electron-beam pumped UVC emitters
title 2D-GaN/AlN Multiple Quantum Disks/Quantum Well Heterostructures for High-Power Electron-Beam Pumped UVC Emitters
title_full 2D-GaN/AlN Multiple Quantum Disks/Quantum Well Heterostructures for High-Power Electron-Beam Pumped UVC Emitters
title_fullStr 2D-GaN/AlN Multiple Quantum Disks/Quantum Well Heterostructures for High-Power Electron-Beam Pumped UVC Emitters
title_full_unstemmed 2D-GaN/AlN Multiple Quantum Disks/Quantum Well Heterostructures for High-Power Electron-Beam Pumped UVC Emitters
title_short 2D-GaN/AlN Multiple Quantum Disks/Quantum Well Heterostructures for High-Power Electron-Beam Pumped UVC Emitters
title_sort 2d gan aln multiple quantum disks quantum well heterostructures for high power electron beam pumped uvc emitters
topic monolayer thick GaN/AlN multiple quantum wells
III-nitrides
carrier localization
plasma-assisted molecular beam epitaxy
electron-beam pumped UVC emitters
url https://www.mdpi.com/2079-4991/13/6/1077
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