Value recovery from spent lithium-ion batteries: A review on technologies, environmental impacts, economics, and supply chain

The demand for lithium-ion batteries (LIBs) has surged in recent years, owing to their excellent electrochemical performance and increasing adoption in electric vehicles and renewable energy storage. As a result, the expectation is that the primary supply of LIB materials (e.g., lithium, cobalt, and...

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Main Authors: Majid Alipanah, Apurba Kumar Saha, Ehsan Vahidi, Hongyue Jin
Format: Article
Language:English
Published: AIMS Press 2021-12-01
Series:Clean Technologies and Recycling
Subjects:
Online Access:https://www.aimspress.com/article/doi/10.3934/ctr.2021008?viewType=HTML
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author Majid Alipanah
Apurba Kumar Saha
Ehsan Vahidi
Hongyue Jin
author_facet Majid Alipanah
Apurba Kumar Saha
Ehsan Vahidi
Hongyue Jin
author_sort Majid Alipanah
collection DOAJ
description The demand for lithium-ion batteries (LIBs) has surged in recent years, owing to their excellent electrochemical performance and increasing adoption in electric vehicles and renewable energy storage. As a result, the expectation is that the primary supply of LIB materials (e.g., lithium, cobalt, and nickel) will be insufficient to satisfy the demand in the next five years, creating a significant supply risk. Value recovery from spent LIBs could effectively increase the critical materials supply, which will become increasingly important as the number of spent LIBs grows. This paper reviews recent studies on developing novel technologies for value recovery from spent LIBs. The existing literature focused on hydrometallurgical-, pyrometallurgical-, and direct recycling, and their advantages and disadvantages are evaluated in this paper. Techno-economic analysis and life cycle assessment have quantified the economic and environmental benefits of LIB reuse over recycling, highlighting the research gap in LIB reuse technologies. The study also revealed challenges associated with changing battery chemistry toward less valuable metals in LIB manufacturing (e.g., replacing cobalt with nickel). More specifically, direct recycling may be impractical due to rapid technology change, and the economic and environmental incentives for recycling spent LIBs will decrease. As LIB collection constitutes a major cost, optimizing the reverse logistics supply chain is essential for maximizing the economic and environmental benefits of LIB recovery. Policies that promote LIB recovery are reviewed with a focus on Europe and the United States. Policy gaps are identified and a plan for sustainable LIB life cycle management is proposed.
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spelling doaj.art-e796a94201c041a29d72c47a88bedab72022-12-22T03:54:46ZengAIMS PressClean Technologies and Recycling2770-45802021-12-011215218410.3934/ctr.2021008Value recovery from spent lithium-ion batteries: A review on technologies, environmental impacts, economics, and supply chainMajid Alipanah 0Apurba Kumar Saha 1Ehsan Vahidi2Hongyue Jin 31. Department of System and Industrial Engineering, University of Arizona, 1127 E. James E. Rogers Way, Tucson, Arizona 85721, United States1. Department of System and Industrial Engineering, University of Arizona, 1127 E. James E. Rogers Way, Tucson, Arizona 85721, United States2. Department of Mining and Metallurgical Engineering, Mackay School of Earth Sciences and Engineering, University of Nevada, 1664 N. Virginia Street, Reno, Nevada 89557, United States1. Department of System and Industrial Engineering, University of Arizona, 1127 E. James E. Rogers Way, Tucson, Arizona 85721, United StatesThe demand for lithium-ion batteries (LIBs) has surged in recent years, owing to their excellent electrochemical performance and increasing adoption in electric vehicles and renewable energy storage. As a result, the expectation is that the primary supply of LIB materials (e.g., lithium, cobalt, and nickel) will be insufficient to satisfy the demand in the next five years, creating a significant supply risk. Value recovery from spent LIBs could effectively increase the critical materials supply, which will become increasingly important as the number of spent LIBs grows. This paper reviews recent studies on developing novel technologies for value recovery from spent LIBs. The existing literature focused on hydrometallurgical-, pyrometallurgical-, and direct recycling, and their advantages and disadvantages are evaluated in this paper. Techno-economic analysis and life cycle assessment have quantified the economic and environmental benefits of LIB reuse over recycling, highlighting the research gap in LIB reuse technologies. The study also revealed challenges associated with changing battery chemistry toward less valuable metals in LIB manufacturing (e.g., replacing cobalt with nickel). More specifically, direct recycling may be impractical due to rapid technology change, and the economic and environmental incentives for recycling spent LIBs will decrease. As LIB collection constitutes a major cost, optimizing the reverse logistics supply chain is essential for maximizing the economic and environmental benefits of LIB recovery. Policies that promote LIB recovery are reviewed with a focus on Europe and the United States. Policy gaps are identified and a plan for sustainable LIB life cycle management is proposed.https://www.aimspress.com/article/doi/10.3934/ctr.2021008?viewType=HTMLpyrometallurgyhydrometallurgyleachingdesign of experimentdisassemblyreverse supply chainlife cycle assessmenteconomic assessment
spellingShingle Majid Alipanah
Apurba Kumar Saha
Ehsan Vahidi
Hongyue Jin
Value recovery from spent lithium-ion batteries: A review on technologies, environmental impacts, economics, and supply chain
Clean Technologies and Recycling
pyrometallurgy
hydrometallurgy
leaching
design of experiment
disassembly
reverse supply chain
life cycle assessment
economic assessment
title Value recovery from spent lithium-ion batteries: A review on technologies, environmental impacts, economics, and supply chain
title_full Value recovery from spent lithium-ion batteries: A review on technologies, environmental impacts, economics, and supply chain
title_fullStr Value recovery from spent lithium-ion batteries: A review on technologies, environmental impacts, economics, and supply chain
title_full_unstemmed Value recovery from spent lithium-ion batteries: A review on technologies, environmental impacts, economics, and supply chain
title_short Value recovery from spent lithium-ion batteries: A review on technologies, environmental impacts, economics, and supply chain
title_sort value recovery from spent lithium ion batteries a review on technologies environmental impacts economics and supply chain
topic pyrometallurgy
hydrometallurgy
leaching
design of experiment
disassembly
reverse supply chain
life cycle assessment
economic assessment
url https://www.aimspress.com/article/doi/10.3934/ctr.2021008?viewType=HTML
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AT apurbakumarsaha valuerecoveryfromspentlithiumionbatteriesareviewontechnologiesenvironmentalimpactseconomicsandsupplychain
AT ehsanvahidi valuerecoveryfromspentlithiumionbatteriesareviewontechnologiesenvironmentalimpactseconomicsandsupplychain
AT hongyuejin valuerecoveryfromspentlithiumionbatteriesareviewontechnologiesenvironmentalimpactseconomicsandsupplychain