Direct detection of Rydberg–Rydberg millimeter-wave transitions in a buffer gas cooled molecular beam

Millimeter-wave transitions between molecular Rydberg states (n ∼ 35) of barium monofluoride are directly detected via Free Induction Decay (FID). Two powerful technologies are used in combination: Chirped-Pulse millimeter-Wave (CPmmW) spectroscopy and a buffer gas cooled molecular beam photoablatio...

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Bibliographic Details
Main Authors: Patterson, David, Muenter, John S., Zhou, Yan, Grimes, David Darrah, Barnum, Timothy James, Coy, Stephen, Klein, Ethan A., Field, Robert W
Other Authors: Massachusetts Institute of Technology. Department of Chemistry
Format: Article
Language:en_US
Published: Elsevier 2016
Online Access:http://hdl.handle.net/1721.1/105273
https://orcid.org/0000-0003-2786-6405
https://orcid.org/0000-0002-5567-7890
https://orcid.org/0000-0002-9363-9844
https://orcid.org/0000-0002-6991-683X
https://orcid.org/0000-0002-7609-4205