Förster resonance energy transfer, absorption and emission spectra in multichromophoric systems. II. Hybrid cumulant expansion

We develop a hybrid cumulant expansion method to account for the system-bath entanglement in the emission spectrum in the multi-chromophoric Förster transfer rate. In traditional perturbative treatments, the emission spectrum is usually expanded with respect to the system-bath coupling term in both...

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Bibliographic Details
Main Authors: Ma, Jian, Moix, Jeremy, Cao, Jianshu
Other Authors: Massachusetts Institute of Technology. Department of Chemistry
Format: Article
Language:en_US
Published: American Institute of Physics (AIP) 2017
Online Access:http://hdl.handle.net/1721.1/110442
https://orcid.org/0000-0001-7616-7809